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    Paraffin-enabled graphene transfer

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    Type
    Article
    Authors
    Leong, Wei Sun cc
    Wang, Haozhe cc
    Yeo, Jingjie cc
    Martin-Martinez, Francisco J. cc
    Zubair, Ahmad cc
    Shen, Pin-Chun
    Mao, Yunwei
    Palacios, Tomas
    Buehler, Markus J.
    Hong, Jin-Yong
    Kong, Jing
    KAUST Grant Number
    OSR-2015-CRG4-2634
    Date
    2019-02-20
    Permanent link to this record
    http://hdl.handle.net/10754/678661
    
    Metadata
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    Abstract
    The performance and reliability of large-area graphene grown by chemical vapor deposition are often limited by the presence of wrinkles and the transfer-process-induced polymer residue. Here, we report a transfer approach using paraffin as a support layer, whose thermal properties, low chemical reactivity and non-covalent affinity to graphene enable transfer of wrinkle-reduced and clean large-area graphene. The paraffin-transferred graphene has smooth morphology and high electrical reliability with uniform sheet resistance with ~1% deviation over a centimeter-scale area. Electronic devices fabricated on such smooth graphene exhibit electrical performance approaching that of intrinsic graphene with small Dirac points and high carrier mobility (hole mobility = 14,215 cm2 V−1 s−1; electron mobility = 7438 cm2 V−1 s−1), without the need of further annealing treatment. The paraffin-enabled transfer process could open realms for the development of high-performance ubiquitous electronics based on large-area two-dimensional materials.
    Citation
    Leong, W. S., Wang, H., Yeo, J., Martin-Martinez, F. J., Zubair, A., Shen, P.-C., … Kong, J. (2019). Paraffin-enabled graphene transfer. Nature Communications, 10(1). doi:10.1038/s41467-019-08813-x
    Sponsors
    J.K. acknowledges the support from AFOSR FATE MURI, Grant No. FA9550-15-1-0514, NSF DMR/ECCS-1509197, the Center for Energy Efficient Electronics Science (NSF Award 0939514), the King Abdullah University of Science and Technology (No. OSR-2015-CRG4-2634), and U.S. Army Research Office through the MIT Institute for Soldier Nanotechnologies (Grant No. 023674). J.-Y.H. acknowledges the support from Korea Research Institute of Chemical Technology (KRICT) project no. KK1801-G01 and the Basic Science Research Program through the National Research Foundation of Korea (NRF) funded by the Ministry of Education (NRF-2017R1C1B2007153). J.Y., F.J.M.-M, and M.J.B also acknowledge support from AFOSR FATE MURI, Grant No. FA9550-15-1-0514 and the US Department of Defense, Office of Naval Research (N00014-16-1-233). The work is partially performed at MIT Microsystems Technology Laboratories (MTL) and Center for Nanoscale Systems (CNS), Harvard University. Computational simulations were performed on the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by the National Science Foundation grant number ACI-1053575, the MIT Engaging Cluster, Singapore's A* STAR Computational Resource Centre, and Singapore's National Supercomputing Centre.
    Publisher
    NATURE PUBLISHING GROUP
    Journal
    NATURE COMMUNICATIONS
    DOI
    10.1038/s41467-019-08813-x
    PubMed ID
    30787292
    PubMed Central ID
    PMC6382797
    Additional Links
    http://www.nature.com/articles/s41467-019-08813-x
    ae974a485f413a2113503eed53cd6c53
    10.1038/s41467-019-08813-x
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