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    Sodium pre-intercalated carbon/V2O5 constructed by sustainable sodium lignosulfonate for stable cathodes in zinc ion batteries: A comprehensive study.

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    ChemSusChem - 2022 - Chen - Sodium pre‐intercalated carbon V2O5 constructed by sustainable sodium lignosulfonate for stable.pdf
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    Type
    Article
    Authors
    Chen, Junli
    Zhang, Wenli
    Zhang, Xiaojun
    Li, Ziyan
    Ma, Jianhui
    Zhao, Lei
    Jian, Wenbin
    Chen, Suli
    Yin, Jian
    Lin, Xuliang
    Qin, Yanlin
    Qiu, Xueqing
    KAUST Department
    Physical Science and Engineering (PSE) Division
    Material Science and Engineering Program
    Date
    2022-05-06
    Embargo End Date
    2023-05-06
    Permanent link to this record
    http://hdl.handle.net/10754/676664
    
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    Abstract
    Aqueous zinc ion battery (AZIB) has been widely investigated in recent years because of its advantages of green, safe and abundant raw materials. It is necessary to continue to study how to prepare cathode materials with excellent performance and high cycling stability toward future commercialization. In this work, we proposed a strategy that uses sodium lignosulfonate as both carbon and sodium source to obtain a sodium pre-intercalated vanadium oxide/carbon (VO/LSC) composite as the cathode of AZIB. The carbon matrix could improve the electronic conductivity of vanadium oxide, while the sodium lignosulfonate can provide sodium ions pre-intercalated into the layered vanadium oxide simultaneously. Through this strategy, we obtained a vanadium-based cathode materials with high stability and excellent rate capability. The VO/LSC cathode delivered high capacities of 350 and 112.8 mAh g -1 at 0.1 and 4.0 A g -1 resepectively. We selected zinc sulfate and zinc trifluoromethyl sulfonate as electrolytes respectively, and analyzed the influence of electrolytes on the performance of VO/LSC. What's more, we used the oxygen in the environment to oxidize the low-priced vanadium oxide to achieve a self-charging AZIB. This paper provide a valuable strategy for the design of vanadium-base cathode material for AZIB, which can broaden the research and application of AZIB.
    Citation
    Chen, J., Zhang, W., Zhang, X., Li, Z., Ma, J., Zhao, L., Jian, W., Chen, S., Yin, J., Lin, X., Qin, Y., & Qiu, X. (2022). Sodium pre-intercalated carbon/V2O5 constructed by sustainable sodium lignosulfonate for stable cathodes in zinc ion batteries: A comprehensive study. ChemSusChem. Portico. https://doi.org/10.1002/cssc.202200732
    Sponsors
    The authors acknowledge the financial support from the National Natural Science Foundation of China (22108044, 22078069), the Guangdong Basic and Applied Basic Research Foundation (No.2019B151502038),the Research and Development Program in Key Fields of Guangdong Province (2020B1111380002),the financial support from the Guangdong Provincial Key Laboratory of Plant Resources Biorefinery (2021GDKLPRB07).
    Publisher
    Wiley
    Journal
    ChemSusChem
    DOI
    10.1002/cssc.202200732
    PubMed ID
    35522223
    Additional Links
    https://onlinelibrary.wiley.com/doi/10.1002/cssc.202200732
    ae974a485f413a2113503eed53cd6c53
    10.1002/cssc.202200732
    Scopus Count
    Collections
    Articles; Physical Science and Engineering (PSE) Division; Material Science and Engineering Program

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