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    Importance of small loops within PIM-1 topology on gas separation selectivity in thin film composite membranes

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    Type
    Article
    Authors
    Foster, Andrew B. cc
    Beal, Joseph L. cc
    Tamaddondar, Marzieh
    Luque-Alled, Jose Miguel
    Robertson, Ben
    Mathias, Michael
    Gorgojo, Patricia cc
    Budd, Peter M. cc
    Date
    2021
    Permanent link to this record
    http://hdl.handle.net/10754/672184
    
    Metadata
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    Abstract
    Studies of blends of topologically distinct samples of the polymer of intrinsic microporosity PIM-1 provide, for the CO$^{2}/N$_{2} gas pair, insight into the optimum loop topology required for high selectivity and permeance of thin film composite (TFC) membranes.
    Citation
    Foster, A. B., Beal, J. L., Tamaddondar, M., Luque-Alled, J. M., Robertson, B., Mathias, M., … Budd, P. M. (2021). Importance of small loops within PIM-1 topology on gas separation selectivity in thin film composite membranes. Journal of Materials Chemistry A. doi:10.1039/d1ta03712a
    Sponsors
    P. M. B., M. T. and A. B. F. would like to thank the support of Programme Grant EP/M01486X/1 (SynFabFun) funded by the Engineering and Physical Sciences Research Council (EPSRC). We thank Emma Enston, Anne Davies, Martin Jennings and Teruo Hashimoto for their assistance in obtaining the MALDITOF mass spectra, elemental analysis and TEM analysis, respectively. We thank Prof. Ingo Pinnau (King Abdullah University of Science and Technology, Saudi Arabia) for kindly providing the porous polyacrylonitrile (PAN) membrane (Sepro PA350 ultrafiltration membrane) used in preparation of TFC membranes.
    Publisher
    Royal Society of Chemistry (RSC)
    Journal
    JOURNAL OF MATERIALS CHEMISTRY A
    DOI
    10.1039/d1ta03712a
    Additional Links
    http://xlink.rsc.org/?DOI=D1TA03712A
    ae974a485f413a2113503eed53cd6c53
    10.1039/d1ta03712a
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