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dc.contributor.authorCan Sener, Serife E.
dc.contributor.authorThomas, Valerie M.
dc.contributor.authorHogan, David E.
dc.contributor.authorMaier, Raina M.
dc.contributor.authorCarbajales-Dale, Michael
dc.contributor.authorBarton, Mark D.
dc.contributor.authorKaranfil, Tanju
dc.contributor.authorCrittenden, John C.
dc.contributor.authorAmy, Gary L.
dc.date.accessioned2021-08-29T07:18:01Z
dc.date.available2021-08-29T07:18:01Z
dc.date.issued2021-08-24
dc.date.submitted2021-05-05
dc.identifier.citationCan Sener, S. E., Thomas, V. M., Hogan, D. E., Maier, R. M., Carbajales-Dale, M., Barton, M. D., … Amy, G. L. (2021). Recovery of Critical Metals from Aqueous Sources. ACS Sustainable Chemistry & Engineering. doi:10.1021/acssuschemeng.1c03005
dc.identifier.issn2168-0485
dc.identifier.issn2168-0485
dc.identifier.doi10.1021/acssuschemeng.1c03005
dc.identifier.urihttp://hdl.handle.net/10754/670801
dc.description.abstractCritical metals, identified from supply, demand, imports, and market factors, include rare earth elements (REEs), platinum group metals, precious metals, and other valuable metals such as lithium, cobalt, nickel, and uranium. Extraction of metals from U.S. saline aqueous, emphasizing saline, sources is explored as an alternative to hardrock ore mining. Potential aqueous sources include seawater, desalination brines, oil- and gas-produced waters, geothermal aquifers, and acid mine drainage, among others. A feasibility assessment reveals opportunities for recovery of lithium, strontium, magnesium, and several REEs from select sources, in quantities significant for U.S. manufacturing and for reduction of U.S. reliance on international supply chains. This is a conservative assessment given that water quality data are lacking for a significant number of critical metals in certain sources. The technology landscape for extraction and recovery of critical metals from aqueous sources is explored, identifying relevant processes along with knowledge gaps. Our analysis indicates that aqueous mining would result in much lower environmental impacts on water, air, and land than ore mining. Preliminary assessments of the economics and energy consumption of recovery show potential for recovery of critical metals.
dc.description.sponsorshipThis work was supported in part by the National Institute of Environmental and Health Sciences (NIEHS) Superfund Program (SRP) Grant P42 ES004940.
dc.publisherAmerican Chemical Society (ACS)
dc.relation.urlhttps://pubs.acs.org/doi/10.1021/acssuschemeng.1c03005
dc.relation.urlhttps://www.ncbi.nlm.nih.gov/pmc/articles/PMC8580379
dc.rightsThis document is the Accepted Manuscript version of a Published Work that appeared in final form in [JournalTitle], copyright © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see [ArticleLink].
dc.rightsThis file is an open access version redistributed from: https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8580379
dc.titleRecovery of Critical Metals from Aqueous Sources
dc.typeArticle
dc.contributor.departmentEnvironmental Science and Engineering Program
dc.contributor.departmentWater Desalination and Reuse Research Center (WDRC)
dc.contributor.departmentBiological and Environmental Science and Engineering (BESE) Division
dc.identifier.journalACS Sustainable Chemistry & Engineering
dc.rights.embargodate2022-08-24
dc.eprint.versionPost-print
dc.contributor.institutionDepartment of Environmental Engineering and Earth Sciences, Clemson University, 342 Computer Court, Anderson, South Carolina 29625, United States
dc.contributor.institutionH. Milton Stewart School of Industrial and Systems Engineering, and School of Public Policy, Georgia Institute of Technology, 755 Ferst Drive NW, Atlanta, Georgia 30332, United States
dc.contributor.institutionDepartment of Environmental Science, University of Arizona, 1177 E Fourth Street, Tucson, Arizona 85721, United States
dc.contributor.institutionDepartment of Geosciences, University of Arizona, 1040 E. Fourth Street, Tucson, Arizona 85721, United States
dc.contributor.institutionSchool of Civil and Environmental Engineering, Georgia Institute of Technology, 790 Atlantic Drive, Atlanta, Georgia 30332, United States
kaust.personAmy, Gary L.
dc.date.accepted2021-08-09
refterms.dateFOA2022-08-24T00:00:00Z
dc.date.published-online2021-08-24
dc.date.published-print2021-09-06


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