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    Recent Advances on Transition Metal Dichalcogenides for Electrochemical Energy Conversion

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    Name:
    MS-Review_AM.pdf
    Size:
    2.474Mb
    Format:
    PDF
    Description:
    Accepted manuscript
    Embargo End Date:
    2022-08-18
    Download
    Type
    Article
    Authors
    Wu, Xin
    Zhang, Huabin cc
    Zhang, Jian
    Lou, Xiong Wen (David)
    KAUST Department
    KAUST Catalysis Center (KCC), Physical Sciences and Engineering Division King Abdullah University of Science and Technology (KAUST) Thuwal 23955–6900 Saudi Arabia
    Physical Science and Engineering (PSE) Division
    Date
    2021-08-18
    Online Publication Date
    2021-08-18
    Print Publication Date
    2021-09
    Embargo End Date
    2022-08-18
    Submitted Date
    2020-12-12
    Permanent link to this record
    http://hdl.handle.net/10754/670690
    
    Metadata
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    Abstract
    Transition metal dichalcogenides (TMDCs) hold great promise for electrochemical energy conversion technologies in view of their unique structural features associated with the layered structure and ultrathin thickness. Because the inert basal plane accounts for the majority of a TMDC's bulk, activation of the basal plane sites is necessary to fully exploit the intrinsic potential of TMDCs. Here, recent advances on TMDCs-based hybrids/composites with greatly enhanced electrochemical activity are reviewed. After a summary of the synthesis of TMDCs with different sizes and morphologies, comprehensive in-plane activation strategies are described in detail, mainly including in-plane-modification-induced phase transformation, surface-layer modulation, and interlayer modification/coupling. Simultaneously, the underlying mechanisms for improved electrochemical activities are highlighted. Finally, the strategic evaluation on further research directions of TMDCs in-plane activation is featured. This work would shed some light on future design trends of TMDCs-based functional materials for electrochemical energy-related applications.
    Citation
    Wu, X., Zhang, H., Zhang, J., & Lou, X. W. (David). (2021). Recent Advances on Transition Metal Dichalcogenides for Electrochemical Energy Conversion. Advanced Materials, 2008376. doi:10.1002/adma.202008376
    Sponsors
    This work was supported by NSFC (21773242, 21935010), the Strategic Priority Research Program of the Chinese Academy of Sciences (XDB20000000), National Key Research and Development Program of China (2018YFA0208600), and King Abdullah University of Science and Technology. X.W.L. acknowledges the funding support from the Ministry of Education of Singapore through the Academic Research Fund (AcRF) Tier-2 grant (MOE2019-T2-2-049).
    Publisher
    Wiley
    Journal
    Advanced Materials
    DOI
    10.1002/adma.202008376
    Additional Links
    https://onlinelibrary.wiley.com/doi/10.1002/adma.202008376
    ae974a485f413a2113503eed53cd6c53
    10.1002/adma.202008376
    Scopus Count
    Collections
    Articles; Physical Science and Engineering (PSE) Division

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