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dc.contributor.authorGuo, Jing
dc.contributor.authorZhang, Wenli
dc.contributor.authorYin, Jun
dc.contributor.authorZhu, Yunpei
dc.contributor.authorMohammed, Zyad O. F.
dc.contributor.authorAlshareef, Husam N.
dc.date.accessioned2021-08-03T13:14:20Z
dc.date.available2021-08-03T13:14:20Z
dc.date.issued2021-08-12
dc.date.submitted2021-06-06
dc.identifier.citationGuo, J., Zhang, W., Yin, J., Zhu, Y., Mohammed, Z. O. F., & Alshareef, H. N. (2021). Zincophilic Laser Scribed Graphene Interlayer for Homogeneous Zinc Deposition and Stable Zinc Ion Batteries. Energy Technology. doi:10.1002/ente.202100490
dc.identifier.issn2194-4288
dc.identifier.issn2194-4296
dc.identifier.doi10.1002/ente.202100490
dc.identifier.urihttp://hdl.handle.net/10754/670385
dc.description.abstractZinc metal is an important anode material for next-generation energy storage systems. Unfortunately, uncontrollable dendrite growth caused by non-uniform Zn nucleation during the plating process severely restricts their practical applications. Herein, a nitrogen-doped 3D laser scribed graphene (NLSG) with a large surface area and uniform distribution of nucleation sites is used as the interlayer to control Zn nucleation behavior and suppress Zn dendrite growth. The N-containing functional groups in the carbon matrix are highly zincophilic, which can induces uniform nucleation of Zn and guides homogenous Zn deposition. Meanwhile, the large specific area could effectively decrease the local current density, which is more favorable for highly reversible Zn plating/stripping. Benefiting from the superior property, the NLSG demonstrates improved electrochemical performance with high Coulombic efficiency (99.4%) and enhanced cycling performance (200 h). Compared with the bare Zn anodes, the NLSG coated Zn//MnO2 battery demonstrated higher capacity retention (72.3% vs. 59.3%) after 1200 cycles.
dc.publisherWiley
dc.relation.urlhttps://onlinelibrary.wiley.com/doi/10.1002/ente.202100490
dc.rightsArchived with thanks to Energy Technology
dc.titleZincophilic Laser Scribed Graphene Interlayer for Homogeneous Zinc Deposition and Stable Zinc Ion Batteries
dc.typeArticle
dc.contributor.departmentFunctional Nanomaterials and Devices Research Group
dc.contributor.departmentMaterial Science and Engineering Program
dc.contributor.departmentPhysical Science and Engineering (PSE) Division
dc.identifier.journalEnergy Technology
dc.rights.embargodate2022-07-29
dc.eprint.versionPost-print
kaust.personGuo, Jing
kaust.personZhang, Wenli
kaust.personYin, Jun
kaust.personZhu, Yunpei
kaust.personMohammed, Zyad O. F.
kaust.personAlshareef, Husam N.
dc.date.accepted2021-07-12
refterms.dateFOA2021-08-03T13:15:18Z
dc.date.published-online2021-08-12
dc.date.published-print2021-10


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