Show simple item record

dc.contributor.authorCheng, Qingpeng
dc.contributor.authorLiu, Yunhao
dc.contributor.authorLyu, Shuaishuai
dc.contributor.authorTian, Ye
dc.contributor.authorMa, Qingxiang
dc.contributor.authorLi, Xingang
dc.date.accessioned2021-07-08T06:50:31Z
dc.date.available2021-07-08T06:50:31Z
dc.date.issued2021-06-04
dc.date.submitted2020-12-28
dc.identifier.citationCheng, Q., Liu, Y., Lyu, S., Tian, Y., Ma, Q., & Li, X. (2021). Manipulating metal-support interactions of metal catalysts for Fischer-Tropsch synthesis. Chinese Journal of Chemical Engineering. doi:10.1016/j.cjche.2021.05.013
dc.identifier.issn1004-9541
dc.identifier.doi10.1016/j.cjche.2021.05.013
dc.identifier.urihttp://hdl.handle.net/10754/670078
dc.description.abstractFor supported metal catalyst systems, the impact on catalysis originates from the interaction between metal nanoparticles and their support. Metal-support interactions (MSI) can change electronic properties, geometric morphologies, or chemical compositions of metal nanoparticles to make active sites have specific properties and catalytic activities. Fischer-Tropsch synthesis (FTS) is one of the most effective ways to convert cheap non-petroleum-based carbon sources into high value-added chemicals or ultra-clean liquid fuels. In this review, we summarize and classify the impact of MSI on the catalytic activity, selectivity and stability of FTS catalysts. The strategies to tune MSI are introduced in detail, and the recent development of high-efficiency FTS catalysts through the manipulation of SMI strategies has been highlighted. It is emphasized that the active metal sites, which are endowed with special functions by MSI, can change the strength of adsorption bond of adsorbates, consequently controlling the product distribution.
dc.description.sponsorshipThe authors are grateful for financial support from the National Natural Science Foundation of China (21676182 and 21476159), the Program for Introducing Talents of Discipline to Universities of China (No. BP0618007), State Key Laboratory of High-efficiency Utilization of Coal and Green Chemical Engineering (2020-KF-26) and open foundation of State Key Laboratory of Chemical Engineering (SKL-ChE-20B01).
dc.publisherElsevier BV
dc.relation.urlhttps://linkinghub.elsevier.com/retrieve/pii/S1004954121002445
dc.rightsNOTICE: this is the author’s version of a work that was accepted for publication in Chinese Journal of Chemical Engineering. Changes resulting from the publishing process, such as peer review, editing, corrections, structural formatting, and other quality control mechanisms may not be reflected in this document. Changes may have been made to this work since it was submitted for publication. A definitive version was subsequently published in Chinese Journal of Chemical Engineering, [, , (2021-06-04)] DOI: 10.1016/j.cjche.2021.05.013 . © 2021. This manuscript version is made available under the CC-BY-NC-ND 4.0 license http://creativecommons.org/licenses/by-nc-nd/4.0/
dc.titleManipulating metal-support interactions of metal catalysts for Fischer-Tropsch synthesis
dc.typeArticle
dc.contributor.departmentAdvanced Membranes and Porous Materials Research Center
dc.contributor.departmentPhysical Science and Engineering (PSE) Division
dc.identifier.journalChinese Journal of Chemical Engineering
dc.rights.embargodate2023-06-04
dc.eprint.versionPost-print
dc.contributor.institutionCollaborative Innovation Center of Chemical Science and Engineering (Tianjin), State Key Laboratory of Chemical Engineering, Tianjin Key Laboratory of Applied Catalysis Science and Technology, School of Chemical Engineering and Technology, Tianjin University, Tianjin 300072, China
dc.contributor.institutionState Key Laboratory of High-efficiency Coal Utilization and Green Chemical Engineering, Ningxia University, Yinchuan 750021, China
dc.contributor.institutionSchool of Chemical and Biological Engineering, Lanzhou Jiaotong University, Lanzhou 730070, China
kaust.personCheng, Qingpeng
dc.date.accepted2021-05-18
dc.identifier.eid2-s2.0-85108979096
dc.date.published-online2021-06-04
dc.date.published-print2021-07


This item appears in the following Collection(s)

Show simple item record