One-step conversion of crude oil to light olefins using a multi-zone reactor
AuthorsAlabdullah, Mohammed A.
Rodriguez Gomez, Alberto
Chowdhury, Abhishek Dutta
Kulkarni, Shekhar Rajabhau
Ali, Ola S.
KAUST DepartmentBiological and Environmental Sciences and Engineering (BESE) Division
Chemical Engineering Program
Clean Combustion Research Center
Combustion and Pyrolysis Chemistry (CPC) Group
Imaging and Characterization Core Lab
KAUST Catalysis Center (KCC)
Physical Science and Engineering (PSE) Division
Saudi Aramco, Chemicals R&D Lab at KAUST, Research and Development Center, Thuwal, Saudi Arabia.
Technology Transfer and Innovation
Embargo End Date2021-08-25
Permanent link to this recordhttp://hdl.handle.net/10754/667715
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AbstractWith the demand for gasoline and diesel expected to decline in the near future, crude-to-chemicals technologies have the potential to become the most important processes in the petrochemical industry. This trend has triggered intense research to maximize the production of light olefins and aromatics at the expense of fuels, which calls for disruptive processes able to transform crude oil to chemicals in an efficient and environmentally friendly way. Here we propose a catalytic reactor concept consisting of a multi-zone fluidized bed that is able to perform several refining steps in a single reactor vessel. This configuration allows for in situ catalyst stripping and regeneration, while the incorporation of silicon carbide in the catalyst confers it with improved physical, mechanical and heat-transport properties. As a result, this reactor–catalyst combination has shown stable conversion of untreated Arabian Light crude into light olefins with yields per pass of over 30 wt% with a minimum production of dry gas.
CitationAlabdullah, M., Rodriguez-Gomez, A., Shoinkhorova, T., Dikhtiarenko, A., Chowdhury, A. D., Hita, I., … Gascon, J. (2021). One-step conversion of crude oil to light olefins using a multi-zone reactor. Nature Catalysis. doi:10.1038/s41929-021-00580-7
SponsorsWe acknowledge Saudi Aramco for financial support. Y. Saih, S. Telalovic and L. E. Gevers are gratefully acknowledged for technical support and S. Ramirez Cherbuy for the artwork design.