Single-atom nickel terminating sp2 and sp3 nitride in polymeric carbon nitride for visible-light photocatalytic overall water splitting

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Article
Authors
Li, Yanrui
Wang, Yiqing
Dong, Chung-Li cc
Huang, Yu-Cheng
Chen, Jie
Zhang, Zhen
Meng, Fanqi
Zhang, Qinghua
Huangfu, Yiliang
Zhao, Daming
Gu, Lin cc
Shen, Shaohua cc
KAUST Department
King Abdullah University of Science and Technology
Date
2021
Submitted Date
2020-12-30
Permanent link to this record
http://hdl.handle.net/10754/667244

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Abstract
Single-atom Ni terminating agent is introduced to coordinate with sp$^{2}$ or sp$^{3}$ N atoms in the heptazine units of PCN, realizing visible-light photocatalytic overall water splitting to H$_{2}$O$_{2}$ and H$_{2}$ without additional cocatalyst.
Citation
Li, Y., Wang, Y., Dong, C.-L., Huang, Y.-C., Chen, J., Zhang, Z., … Shen, S. (2021). Single-atom nickel terminating sp2 and sp3 nitride in polymeric carbon nitride for visible-light photocatalytic overall water splitting. Chemical Science. doi:10.1039/d0sc07093a
Sponsors
This work was supported by the National Natural Science Foundation of China (51961165103 and 21875183), the National Key Research and Development Program of China (2017YFE0193900), the National Program for Support of Top notch Young Professionals, the “Fundamental Research Funds for the Central Universities”, the Project Supported by the Natural Science Basic Research Plan in Shaanxi Province of China (2018JQ2028), the China Postdoctoral Science Foundation (2018M640981), and “The Youth Innovation Team of Shaanxi Universities”. C.L.D is grateful to MoST for financially supporting this work under contracts MoST 107-2112-M-032-004-MY3 and 108-2218-E-032-003-MY3.
Publisher
Royal Society of Chemistry (RSC)
Journal
Chemical Science
DOI
10.1039/d0sc07093a
Additional Links
http://xlink.rsc.org/?DOI=D0SC07093A
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Except where otherwise noted, this item's license is described as This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.