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dc.contributor.authorJolly, Anju
dc.contributor.authorUday, Anjana
dc.contributor.authorGurumurthy, S. C.
dc.contributor.authorShilpa, M. P.
dc.contributor.authorSurabhi, Srivathsava
dc.contributor.authorMundinamani, Shridhar
dc.contributor.authorRamam, Koduri
dc.contributor.authorGedda, Murali
dc.contributor.authorMurari, M. S.
dc.contributor.authorJeong, Jong Ryul
dc.date.accessioned2021-02-04T06:30:38Z
dc.date.available2021-02-04T06:30:38Z
dc.date.issued2021-01-21
dc.date.submitted2020-08-13
dc.identifier.citationJolly, A., Uday, A., Gurumurthy, S. C., Shilpa, M. P., Surabhi, S., Mundinamani, S., … Jeong, J.-R. (2021). Effect of silane/amine-based dopants on polymer-metal interaction of sub-surface silver nanoparticulate films. Journal of Materials Science: Materials in Electronics. doi:10.1007/s10854-020-04995-z
dc.identifier.issn1573-482X
dc.identifier.issn0957-4522
dc.identifier.doi10.1007/s10854-020-04995-z
dc.identifier.urihttp://hdl.handle.net/10754/667212
dc.description.abstractThe optical and morphological properties of the vacuum-evaporated silver (Ag) nanoparticulate films on softened polyvinyl alcohol (PVA) modified with the 3-mercaptopropyl trimethoxysilane (MPTMS) and 3-aminopropyl trimethoxysilane (APTMS) dopants are reported. The topography of the particulate films is characterized by the field-emission scanning electron microscopy. The optical spectra broadening, red-shift, and the increase in the intensity values of the plasmonic resonance peak with the nature of dopant have a strong dependence on the particle size, shape, and inter-particle separation. The conducted experimental optical studies are supported by Finite Difference Time-Domain (FDTD) simulation results. Quantitative analysis of the Fourier-Transform Infrared Spectroscopy (FTIR) and Raman Spectroscopy studies confirm the surface modification of Ag nanoparticulate films on doped PVA substrates. The amount of polymer-metal interaction caused by the strongly interacting silane groups of the dopants and their influence on the morphology and optical properties are discussed.
dc.description.sponsorshipAll authors are greatly indebted to their respective affiliated organizations for their enormous support and facilities. However, they thank Prof. Mohan Rao, Department of Physics, Manipal Institute of Technology, India for facilitating his lab for the experimental work prior to the formation of Nanomaterials and Polymer Physics laboratory, Laboratorio de Nanocompuestos, Departamento de Ingeniería de Materiales (DIMAT), Universidad de Concepción (UdeC), Chile, and Spintronics Materials and Application Lab (SMAL), Chungnam National University, South Korea for simulation works. This work was supported by the Manipal Academy of Higher Education (MIT-2017, 2020), Karnataka and also acknowledges the Fondecyt Project No 3200832, Programa Fondo Nacional de Desarrollo Científico y Tecnológico (FONDECYT) de la Agencia Nacional de Investigación y Desarrollo, Chile.
dc.publisherSpringer Nature
dc.relation.urlhttp://link.springer.com/10.1007/s10854-020-04995-z
dc.rightsThis article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder.
dc.rights.urihttps://creativecommons.org/licenses/by/4.0
dc.titleEffect of silane/amine-based dopants on polymer-metal interaction of sub-surface silver nanoparticulate films
dc.typeArticle
dc.contributor.departmentKAUST Solar Center (KSC)
dc.contributor.departmentPhysical Science and Engineering (PSE) Division
dc.identifier.journalJournal of Materials Science: Materials in Electronics
dc.eprint.versionPublisher's Version/PDF
dc.contributor.institutionNanomaterials and Polymer Physics Lab, Department of Physics, Manipal Institute of Technology, Manipal Academy of Higher Education, Manipal, 576104, India
dc.contributor.institutionFunctional Materials Group, Institute for Future Transport and Cities, Coventry University, Coventry, CV1 5FB, United Kingdom
dc.contributor.institutionInstitute of Physics II, University of Cologne, 50923, Köln, Germany
dc.contributor.institutionLaboratorio de Nanocompuestos, Departamento de Ingeniería de Materiales (DIMAT), Facultad de Ingeniería (FI), Universidad de Concepción (UdeC), Concepción, Chile
dc.contributor.institutionDepartment of Materials Science and Engineering, Graduate School of Energy Science and Technology, Chungnam National University, Daejeon, 34134, South Korea
dc.contributor.institutionDepartment of Physics, Siddaganga Institute of Technology, Tumakuru, 572 103, Karnataka, India
dc.contributor.institutionDST Purse Lab, Mangalore University, Mangalagangotri, 574 199, India
kaust.personGedda, Murali
dc.date.accepted2020-11-28
dc.identifier.eid2-s2.0-85099904317
refterms.dateFOA2021-02-04T06:31:15Z
dc.date.published-online2021-01-21
dc.date.published-print2021-02


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This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder.
Except where otherwise noted, this item's license is described as This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder.