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    Liquid nanoparticles: manipulating the nucleation and growth of nanoscale droplets.

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    Name:
    liquid nanoparticles.pdf
    Size:
    1.003Mb
    Format:
    PDF
    Description:
    Accepted manuscript
    Embargo End Date:
    2021-11-16
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    Type
    Article
    Authors
    Wang, Ruoxu
    Han, Fei
    Chen, Bo
    Liu, Lingmei
    Wang, Shaoyan
    Zhang, Hua
    Han, Yu cc
    Chen, Hongyu
    KAUST Department
    Advanced Membranes and Porous Materials Research Center
    Chemical Science Program
    Nanostructured Functional Materials (NFM) laboratory
    Physical Science and Engineering (PSE) Division
    Date
    2020-11-15
    Embargo End Date
    2021-11-16
    Submitted Date
    2020-09-15
    Permanent link to this record
    http://hdl.handle.net/10754/666023
    
    Metadata
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    Abstract
    By manipulating the nucleation and growth of solid materials, the synthesis of various sophisticated nanostructures has been achieved. Similar methodology, if applied to liquid, could enable the mass-production and control of ultra-small droplets at the scale of nanoparticles (10 -18  L or below). It would be highly desirable since droplets plays a fundamental role in numerous applications. Here we present a general strategy to synthesize and manipulate nanoscale droplets, similar to what has been done to solid nanoparticles in the classis solution-synthesis. It was achieved by a solute-induced phase separation which initiates the nucleation of droplets from a homogeneous solution. These liquid nanoparticles have great potentials to be manipulated like their solid counterparts, borrowing from the vast methodologies of nanoparticle synthesis, such as burst nucleation, seeded growth and co-precipitations. LNPs also serve as a general synthetic platform, to fabricate nanoreactors, drug-loaded carriers, and other hollow nanostructures with a variety of shell materials.
    Citation
    Wang, R., Han, F., Chen, B., Liu, L., Wang, S., Zhang, H., … Chen, H. (2020). Liquid nanoparticles: manipulating the nucleation and growth of nanoscale droplets. Angewandte Chemie International Edition. doi:10.1002/anie.202012564
    Sponsors
    The authors thank the Facility for Analysis Characterisation Testing and Simulation of the Nanyang Technological University for access to the facilities. This work is support by the National Natural Science Foundation of China (No. 21673117), Recruitment Program of Global Experts, Jiangsu Provincial Foundation for Specially Appointed Professor, Start-up fund of Nanjing Tech University (39837102), and SICAM Fellowship from Jiangsu National Synergetic Innovation Center for Advanced Materials. Ministry of Education Academic Research Fund (AcRF) Tier 1: RG10/16, RG111/15, Singapore. H.Z. thanks the financial support from ITC via Hong Kong Branch of National Precious Metals Material Engineering Research Center (NPMM), and the start-up grant (Project No. 9380100) and grants (Project No. 9610478 and 1886921) in City University of Hong Kong.
    Publisher
    Wiley
    Journal
    Angewandte Chemie (International ed. in English)
    DOI
    10.1002/anie.202012564
    10.1002/ange.202012564
    10.1002/anie.202100087
    10.1002/ange.202100087
    PubMed ID
    33191586
    Additional Links
    https://onlinelibrary.wiley.com/doi/10.1002/anie.202012564
    ae974a485f413a2113503eed53cd6c53
    10.1002/anie.202012564
    Scopus Count
    Collections
    Articles; Advanced Membranes and Porous Materials Research Center; Physical Science and Engineering (PSE) Division; Chemical Science Program

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