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    Shape Control of Metal Halide Perovskite Single Crystals: From Bulk to Nanoscale

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    Name:
    20200828 Manuscript.pdf
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    1.544Mb
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    PDF
    Description:
    Accepted Manuscript
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    Type
    Article
    Authors
    Feng, Anbo
    Jiang, Xiaomei
    Zhang, Xiaoyu cc
    Zheng, Xiaopeng
    Zheng, Weitao
    Mohammed, Omar F. cc
    Chen, Zhaolai cc
    Bakr, Osman cc
    KAUST Department
    Chemical Science Program
    Functional Nanomaterials Lab (FuNL)
    KAUST Catalysis Center (KCC)
    KAUST Solar Center (KSC)
    Material Science and Engineering
    Material Science and Engineering Program
    Physical Science and Engineering (PSE) Division
    Ultrafast Laser Spectroscopy and Four-dimensional Electron Imaging Research Group
    Date
    2020-08-12
    Online Publication Date
    2020-08-12
    Print Publication Date
    2020-09-22
    Embargo End Date
    2021-08-12
    Submitted Date
    2020-05-31
    Permanent link to this record
    http://hdl.handle.net/10754/665675
    
    Metadata
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    Abstract
    Metal halide perovskite (MHP) single crystals are promising candidates for photovoltaics and related optoelectronic devices. They afford optical and charge transport properties superior to those of their polycrystalline counterparts. Despite this advantage, MHP single crystals are less widely adopted. Traditional bulk growth methods do not lend single-crystal MHPs to device integration as readily as their polycrystalline analogues, which are amenable to a multitude of approaches for deposition and growth. Fortunately, diverse shape-control approaches for MHP single crystals have been recently reported, enabling tunable optoelectronic properties and expanding the potential for single-crystal applications. In this review, we summarize recent developments in the shape control of MHP single crystals, including those pertaining to microcrystals, single-crystal thin films, nano/microplates, nano/microrods, and nanocrystals. We highlight strategies for optimizing the synthesis of these crystals to achieve targeted materials properties and device performance. This review aims to guide the future of shape design in MHP single crystals for various optoelectronic applications.
    Citation
    Feng, A., Jiang, X., Zhang, X., Zheng, X., Zheng, W., Mohammed, O. F., … Bakr, O. M. (2020). Shape Control of Metal Halide Perovskite Single Crystals: From Bulk to Nanoscale. Chemistry of Materials, 32(18), 7602–7617. doi:10.1021/acs.chemmater.0c02269
    Sponsors
    The authors acknowledge funding support from Shandong University, KAUST, and Saudi Aramco (Grant No. RGC/3/3543-01-01).
    Publisher
    American Chemical Society (ACS)
    Journal
    Chemistry of Materials
    DOI
    10.1021/acs.chemmater.0c02269
    Additional Links
    https://pubs.acs.org/doi/10.1021/acs.chemmater.0c02269
    ae974a485f413a2113503eed53cd6c53
    10.1021/acs.chemmater.0c02269
    Scopus Count
    Collections
    Articles; Physical Science and Engineering (PSE) Division; Chemical Science Program; Material Science and Engineering Program; KAUST Catalysis Center (KCC); KAUST Solar Center (KSC)

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