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    Understanding the hierarchical assemblies and oil/water separation applications of metal-organic frameworks

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    1-s2.0-S0167732220339180-main.pdf
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    Description:
    Accepted Manuscript
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    Type
    Article
    Authors
    Ali, Nisar
    Bilal, Muhammad
    Khan, Adnan
    Ali, Farman
    Khan, Hamayun
    Khan, Hassnain Abbas cc
    Rasool, Kashif
    Iqbal, Hafiz M.N.
    KAUST Department
    Clean Combustion Research Center
    Physical Science and Engineering (PSE) Division
    Date
    2020-09-13
    Online Publication Date
    2020-09-13
    Print Publication Date
    2020-11
    Embargo End Date
    2022-09-07
    Permanent link to this record
    http://hdl.handle.net/10754/665121
    
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    Abstract
    Considering the growing environmental concern, there is a dire need to understand the persistence of hydrocarbon-based toxic substances, both in pristine and mix forms, in different matrices. Most of these toxic substances pose hazardous threats directly or indirectly to entire living ecosystems. In this context, the uncontrolled or accidental leakage of petrochemicals and/or trace residues from the oilfields or refinery units are considered a rich source of emerging contaminants with a notable potential to damage the water matrices. Thus, effective treatment with standardized measures is of supreme interest to address the environmental pollution, at large, and water insecurity, in particular. Robust remediation measures should be taken to mitigate or at least lower the environmentally related adverse impacts and human-health related threatening concerns of hydrocarbon-based toxic substances. Several of in practice conventional treatments had been old-fashioned, insufficient, and expensive. Herein, we reviewed metal-organic frameworks (MOFs) based innovative approaches to tackle hydrocarbon-based petroleum source contamination. Metal ion or clusters incorporated in organic ligands leads to the formation of one, two-dimensional (2D) or three-dimensional (3D) hierarchy materials so-called “MOFs”. Besides, the bond flexibility between inorganic (metal) and organic polymers) units, intricate synthesis of MOFs with requisite functionalities for oil/water separation. The selection of accurate metal and organic components for the integration of chemically and thermally stable MOF crystals with high porosity is essential, especially to explain oil/water separation applications. This review spotlights to understand the hierarchical assemblies and structural geometries of MOFs, followed by applications in the separation of oil/water mixtures for a safer environment.
    Citation
    Ali, N., Bilal, M., Khan, A., Ali, F., Khan, H., Khan, H. A., … Iqbal, H. M. N. (2020). Understanding the hierarchical assemblies and oil/water separation applications of metal-organic frameworks. Journal of Molecular Liquids, 114273. doi:10.1016/j.molliq.2020.114273
    Sponsors
    Authors are grateful to their representative institutes for providing the literature access.
    Publisher
    Elsevier BV
    Journal
    Journal of Molecular Liquids
    DOI
    10.1016/j.molliq.2020.114273
    Additional Links
    https://linkinghub.elsevier.com/retrieve/pii/S0167732220339180
    ae974a485f413a2113503eed53cd6c53
    10.1016/j.molliq.2020.114273
    Scopus Count
    Collections
    Articles; Physical Science and Engineering (PSE) Division; Clean Combustion Research Center

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