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    High-Performance Perovskite Single-Junction and Textured Perovskite/Silicon Tandem Solar Cells via Slot-Die Coating

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    HHHigh performance.pdf
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    Type
    Article
    Authors
    Subbiah, Anand Selvin
    Isikgor, Furkan Halis cc
    Howells, Calvyn Travis
    de Bastiani, Michele
    Liu, Jiang cc
    Aydin, Erkan
    Furlan, Francesco
    Allen, Thomas
    Xu, Fuzong
    Zhumagali, Shynggys
    Hoogland, Sjoerd
    Sargent, Edward H.
    McCulloch, Iain cc
    De Wolf, Stefaan cc
    KAUST Department
    Chemical Science Program
    KAUST Solar Center (KSC)
    Material Science and Engineering Program
    Physical Science and Engineering (PSE) Division
    Date
    2020-08-11
    Online Publication Date
    2020-08-11
    Print Publication Date
    2020-09-11
    Embargo End Date
    2021-08-11
    Permanent link to this record
    http://hdl.handle.net/10754/664695
    
    Metadata
    Show full item record
    Abstract
    In this work we report perovskite solar cells in the planar p-i-n configuration based on single-step, anti-solvent free, low-temperature (70 oC) slot-die coated methylammonium lead tri-iodide (MAPbI3). The devices are fabricated on hydrophobic PTAA surfaces, using key strategies such as solvent engineering, enhanced ink-substrate dynamics, and surface passivation, enabling a power conversion efficiency (PCE) of 21.8%. We also adapted the technique to achieve the first slot-die coated perovskite/silicon monolithic 2-terminal tandems, achieving a PCE of 23.8% utilizing a textured silicon bottom cell.
    Citation
    Subbiah, A. S., Isikgor, F. H., Howells, C. T., De Bastiani, M., Liu, J., Aydin, E., … De Wolf, S. (2020). High-Performance Perovskite Single-Junction and Textured Perovskite/Silicon Tandem Solar Cells via Slot-Die Coating. ACS Energy Letters. doi:10.1021/acsenergylett.0c01297
    Sponsors
    The authors acknowledge the support of the King Abdullah University of Science and Technology (KAUST) Office of Sponsored Research (OSR) under award no. KAUST OSR-CARF URF/1/3097, as well as funding support from QD Solar, Inc. The authors also thank the members of the KAUST Solar Center operations team for their valuable support. The authors also thank all the previous reports tabulated in Table S5 for the data points compiled in the TOC graphic
    Publisher
    American Chemical Society (ACS)
    Journal
    ACS Energy Letters
    DOI
    10.1021/acsenergylett.0c01297
    Additional Links
    https://pubs.acs.org/doi/10.1021/acsenergylett.0c01297
    ae974a485f413a2113503eed53cd6c53
    10.1021/acsenergylett.0c01297
    Scopus Count
    Collections
    Articles; Physical Science and Engineering (PSE) Division; Chemical Science Program; Material Science and Engineering Program; KAUST Solar Center (KSC)

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