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dc.contributor.authorLiu, Yunling
dc.contributor.authorLi, Jiantang
dc.contributor.authorKan, Liang
dc.contributor.authorLi, Jiyang
dc.contributor.authorEddaoudi, Mohamed
dc.date.accessioned2020-07-16T13:11:10Z
dc.date.available2020-07-16T13:11:10Z
dc.date.issued2020-08-26
dc.date.submitted2020-05-14
dc.identifier.citationLiu, Y., Li, J., Kan, L., Li, J., & Eddaoudi, M. (2020). Quest for Zeolite-like Supramolecular Assemblies: Self-Assembly of Metal-Organic Squares via Directed Hydrogen Bonding. Angewandte Chemie International Edition. doi:10.1002/anie.202006978
dc.identifier.issn1433-7851
dc.identifier.pmid32662153
dc.identifier.doi10.1002/anie.202006978
dc.identifier.urihttp://hdl.handle.net/10754/664243
dc.description.abstractOur conceived approach based on the directed assembly of functional metal-organic squares (MOSs), 4-membered ring (4MR) building units, permitted the construction of two novel zeolite-like supramolecular assemblies (ZSAs), namely [Co 4 (ImDC) 4 (En) 4 ]·9H 2 O·1.5DMF ( ZSA-10 ) and [Co 4 (ImDC) 4 (En) 4 ]·7H 2 O ( ZSA-11 ) (H 3 ImDC = 4,5-imidazoledicarboxylic acid, En = ethylenediamine, DMF = N,N-dimethylformamide). The elected MOSs encompass both trans - and cis -coordinated nodes, offering complementary peripheral functional groups for their directed assembly into zeolite-like topologies via supramolecular hydrogen bonding interactions. Distinctly, ZSA-10 possesses the underling MER zeolite topology and is the only pure MER framework material (without any supporting templates) exhibiting permanent porosity up to now. ZSA-11 has the underlying ABW topology together with one type of narrow channel.
dc.publisherWiley
dc.relation.urlhttps://onlinelibrary.wiley.com/doi/abs/10.1002/anie.202006978
dc.rightsArchived with thanks to Angewandte Chemie (International ed. in English)
dc.titleQuest for Zeolite-like Supramolecular Assemblies: Self-Assembly of Metal-Organic Squares via Directed Hydrogen Bonding.
dc.typeArticle
dc.contributor.departmentAdvanced Membranes and Porous Materials Research Center
dc.contributor.departmentChemical Science Program
dc.contributor.departmentFunctional Materials Design, Discovery and Development (FMD3)
dc.contributor.departmentPhysical Science and Engineering (PSE) Division
dc.identifier.journalAngewandte Chemie
dc.rights.embargodate2021-07-15
dc.eprint.versionPost-print
dc.contributor.institutionJilin UniversityState Key Laboratory of Inorganic Synthesis and Preparative Chemistry 2699 Qianjin Street 130012 Changchun CHINA
dc.contributor.institutionJilin UniversityCollege of Chemistry CHINA
kaust.personEddaoudi, Mohamed
dc.date.accepted2020-07-13
dc.relation.issupplementedbyDOI:10.5517/ccdc.csd.cc1zzc3f
dc.relation.issupplementedbyDOI:10.5517/ccdc.csd.cc1zzc5h
dc.relation.issupplementedbyDOI:10.5517/ccdc.csd.cc1zzc4g
refterms.dateFOA2020-07-16T13:12:36Z
display.relations<b>Is Supplemented By:</b><br/> <ul><li><i>[Dataset]</i> <br/> Liu, Yunling, Li, Jiantang, Kan, Liang, Li, Jiyang, &amp; Eddaoudi, Mohamed. (2020). <i>CCDC 1846425: Experimental Crystal Structure Determination</i> [Data set]. Cambridge Crystallographic Data Centre. https://doi.org/10.5517/CCDC.CSD.CC1ZZC3F. DOI: <a href="https://doi.org/10.5517/ccdc.csd.cc1zzc3f" >10.5517/ccdc.csd.cc1zzc3f</a> HANDLE: <a href="http://hdl.handle.net/10754/665908">10754/665908</a></li><li><i>[Dataset]</i> <br/> Liu, Yunling, Li, Jiantang, Kan, Liang, Li, Jiyang, &amp; Eddaoudi, Mohamed. (2020). <i>CCDC 1846427: Experimental Crystal Structure Determination</i> [Data set]. Cambridge Crystallographic Data Centre. https://doi.org/10.5517/CCDC.CSD.CC1ZZC5H. DOI: <a href="https://doi.org/10.5517/ccdc.csd.cc1zzc5h" >10.5517/ccdc.csd.cc1zzc5h</a> HANDLE: <a href="http://hdl.handle.net/10754/665909">10754/665909</a></li><li><i>[Dataset]</i> <br/> Liu, Yunling, Li, Jiantang, Kan, Liang, Li, Jiyang, &amp; Eddaoudi, Mohamed. (2020). <i>CCDC 1846426: Experimental Crystal Structure Determination</i> [Data set]. Cambridge Crystallographic Data Centre. https://doi.org/10.5517/CCDC.CSD.CC1ZZC4G. DOI: <a href="https://doi.org/10.5517/ccdc.csd.cc1zzc4g" >10.5517/ccdc.csd.cc1zzc4g</a> HANDLE: <a href="http://hdl.handle.net/10754/665911">10754/665911</a></li></ul>
dc.date.published-online2020-08-26
dc.date.published-print2020-10-26


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