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dc.contributor.authorCenker, Emre
dc.contributor.authorBennett, A.
dc.contributor.authorRoberts, W. L.
dc.date.accessioned2020-06-24T07:17:26Z
dc.date.available2020-06-24T07:17:26Z
dc.date.issued2017
dc.identifier.citationE. Cenker, A. Bennett, & W. L. Roberts. (2017). Investigations of the long-term effects of LII on soot and bath gas [Data set]. Taylor & Francis. https://doi.org/10.6084/M9.FIGSHARE.5341276.V1
dc.identifier.doi10.6084/m9.figshare.5341276.v1
dc.identifier.urihttp://hdl.handle.net/10754/663814
dc.description.abstractA combination of high-repetition rate imaging, laser extinction measurements, two-color soot pyrometry imaging, and high-resolution transmission electron microscopy of thermophoretically sampled soot is used to investigate the long-term and permanent effects of rapid heating of in-flame soot during laser-induced incandescence (LII). Experiments are carried out on a laminar non-premixed co-annular ethylene/air flame with various laser fluences. The high-repetition rate images clearly show that the heated and the neighboring laser-border zones undergo a permanent transformation after the laser pulse, and advect vertically with the flow while the permanent marking is preserved. The soot volume fraction at the heated zone reduces due to the sublimation of soot and the subsequent enhanced oxidation. At the laser-border zones, however, optical thickness increases that may be due to thermophoretic forces drawing hot particles towards relatively cooler zones and the rapid compression of the bath gas induced by the pressure waves created by the expansion of the desorbed carbon clusters. Additionally sublimed carbon clusters can condense onto existing particles and contribute to increase of the optical thickness. Time-resolved two-color pyrometry imaging show that the increased temperature of soot both in the heated and neighboring laser-border zones persists for several milliseconds. This can be associated to the increase in the bath-gas temperature, and a change in the wavelength-dependent emissivity of soot particles induced by the thermal annealing of soot. Ex-situ analysis show that the lattice structure of the soot sampled at the laser-border zones tend to change and soot becomes more graphitic. This may be attributed to thermal annealing induced by elevated temperature. Copyright © 2017 American Association for Aerosol Research
dc.publisherfigshare
dc.subjectBiophysics
dc.subject29999 Physical Sciences not elsewhere classified
dc.subjectMicrobiology
dc.subjectPhysiology
dc.subjectBiotechnology
dc.subjectEvolutionary Biology
dc.subject59999 Environmental Sciences not elsewhere classified
dc.subjectEcology
dc.subject20199 Astronomical and Space Sciences not elsewhere classified
dc.titleInvestigations of the long-term effects of LII on soot and bath gas
dc.typeDataset
dc.contributor.departmentClean Combustion Research Center
dc.contributor.departmentKing Abdullah University of Science and Technology (KAUST),Clean Combustion Research Center (CCRC), Thuwal 23955–6900, Saudi Arabia
dc.contributor.departmentPhysical Science and Engineering (PSE) Division
kaust.personCenker, Emre
kaust.personBennett, A.
dc.relation.issupplementtoDOI:10.1080/02786826.2017.1368444
display.relations<b> Is Supplement To:</b><br/> <ul> <li><i>[Article]</i> <br/> Cenker E, Bennett A, Roberts WL (2017) Investigations of the long-term effects of LII on soot and bath gas. Aerosol Science and Technology: 00–00. Available: http://dx.doi.org/10.1080/02786826.2017.1368444.. DOI: <a href="https://doi.org/10.1080/02786826.2017.1368444" >10.1080/02786826.2017.1368444</a> HANDLE: <a href="http://hdl.handle.net/10754/625425">10754/625425</a></li></ul>


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