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    Hydrogenation or Dehydrogenation of N-Containing Heterocycles Catalyzed by a Single Manganese Complex

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    Hydrogenation.pdf
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    Description:
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    Type
    Article
    Authors
    Zubar, Viktoriia
    Borghs, Jannik C.
    Rueping, Magnus cc
    KAUST Department
    Chemical Science Program
    KAUST Catalysis Center (KCC)
    Physical Science and Engineering (PSE) Division
    Date
    2020-05-04
    Online Publication Date
    2020-05-04
    Print Publication Date
    2020-05-15
    Embargo End Date
    2021-05-04
    Submitted Date
    2020-04-10
    Permanent link to this record
    http://hdl.handle.net/10754/662745
    
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    Abstract
    A highly chemoselective base-metal catalyzed hydrogenation and acceptorless dehydrogenation of N-heterocycles is presented. A well-defined Mn complex operates at low catalyst loading (as low as 2 mol %) and under mild reaction conditions. The described catalytic system tolerates various functional groups, and the corresponding reduced heterocycles can be obtained in high yields. Experimental studies indicate a metal-ligand cooperative catalysis mechanism
    Citation
    Zubar, V., Borghs, J. C., & Rueping, M. (2020). Hydrogenation or Dehydrogenation of N-Containing Heterocycles Catalyzed by a Single Manganese Complex. Organic Letters. doi:10.1021/acs.orglett.0c01273
    Sponsors
    This work was financially supported by the King Abdullah University of Science and Technology (KAUST), Saudi Arabia, Office of Sponsored Research (FCC/1/1974).
    Publisher
    American Chemical Society (ACS)
    Journal
    Organic Letters
    DOI
    10.1021/acs.orglett.0c01273
    Additional Links
    https://pubs.acs.org/doi/10.1021/acs.orglett.0c01273
    ae974a485f413a2113503eed53cd6c53
    10.1021/acs.orglett.0c01273
    Scopus Count
    Collections
    Articles; Physical Science and Engineering (PSE) Division; Chemical Science Program; KAUST Catalysis Center (KCC)

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