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    Solution-Processed Mixed-Dimensional Hybrid Perovskite/Carbon Nanotube Electronics.

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    Chun Deposit.pdf
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    Type
    Article
    Authors
    Ma, Chun cc
    Clark, Sarah
    Liu, Zhixiong
    Liang, Liangliang cc
    Firdaus, Yuliar cc
    Tao, Ran cc
    Han, Ali
    Liu, Xiaogang cc
    Li, Lain-Jong cc
    Anthopoulos, Thomas D. cc
    Hersam, Mark C cc
    Wu, Tao cc
    KAUST Department
    KAUST Solar Center (KSC)
    Material Science and Engineering Program
    Mechanical Engineering Program
    Physical Science and Engineering (PSE) Division
    Date
    2020-03-02
    Online Publication Date
    2020-03-02
    Print Publication Date
    2020-04-28
    Embargo End Date
    2021-03-03
    Submitted Date
    2019-10-06
    Permanent link to this record
    http://hdl.handle.net/10754/662383
    
    Metadata
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    Abstract
    Benefiting from their extraordinary physical properties, methylammonium lead halide perovskites (PVKs) have attracted significant attention in optoelectronics. However, the PVK-based devices suffer from low carrier mobility and high operation voltage. Here, we utilize sorted semiconducting single-walled carbon nanotubes (95% s-SWCNTs) to enhance the performance of thin-film transistors (TFTs) based on the mixed-cation perovskite (MA1-xFAx)Pb(I1-xBrx)3, enabling mixed-dimensional solution-processed electronics with high mobility (32.25 cm2/(V s)) and low voltage (∼3 V) operation. The resulting mixed-dimensional PVK/SWCNT TFTs possess ON/OFF ratios on the order of 107, enabling the fabrication of high-gain inverters.
    Citation
    Ma, C., Clark, S., Liu, Z., Liang, L., Firdaus, Y., Tao, R., … Wu, T. (2020). Solution-Processed Mixed-Dimensional Hybrid Perovskite/Carbon Nanotube Electronics. ACS Nano. doi:10.1021/acsnano.9b07888
    Sponsors
    This research was supported by the Materials Research Science and Engineering Center (MRSEC) of Northwestern University (NSFDMR-1720139). This research was supported by Material Science and Engineering (MSE) of King Abdullah University of Science and Technology. T.W. and M.H. conceived and supervised the project. C.M., S.C., L.L., R.T., and A.H. wrote the paper. C.M., Z.L., and A.H. fabricated and characterized the devices. Y.F. performed ellipsometry. S.C. synthesized unsorted and sorted s-SWCNT. L.J.L. provided metallic SWCNTs. All authors discussed the results
    Publisher
    American Chemical Society (ACS)
    Journal
    ACS nano
    DOI
    10.1021/acsnano.9b07888
    PubMed ID
    32119769
    Additional Links
    https://pubs.acs.org/doi/10.1021/acsnano.9b07888
    ae974a485f413a2113503eed53cd6c53
    10.1021/acsnano.9b07888
    Scopus Count
    Collections
    Articles; Physical Science and Engineering (PSE) Division; Material Science and Engineering Program; Mechanical Engineering Program; KAUST Solar Center (KSC)

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