Dark-current reduction accompanied photocurrent enhancement in p-type MnO quantum-dot decorated n-type 2D-MoS2-based photodetector
Roqan, Iman S.
KAUST DepartmentElectron Microscopy
Material Science and Engineering Program
Physical Science and Engineering (PSE) Division
Semiconductor and Material Spectroscopy (SMS) Laboratory
Embargo End Date2021-03-16
Permanent link to this recordhttp://hdl.handle.net/10754/662194
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AbstractA highly crystalline single- or few-layered 2D-MoS2 induces a high dark current, due to which an extremely small photocurrent generated by a few photons can be veiled or distorted. In this report, we show that suppression in the dark current with the enhancement in the photocurrent of a 2D-based photodetector, which is a prerequisite for photoresponse enhancement, can be achieved by constructing an ideal p-n junction based on functionalizing n-type 2D-MoS2 with p-type quantum dots (QDs). Highly crystalline solution-processed manganese oxide QDs (MnO QDs) are synthesized via the pulsed femtosecond laser ablation technique in ethanol. The ablated MnO QDs are spray-coated on an exfoliated 2D-MoS2 substrate with interdigitated Au electrodes through N2-assisted spraying. In the resulting MnO QD-decorated 2D-MoS2 photodetector with a heterojunction, dark current is reduced and is accompanied by photocurrent enhancement, thereby markedly improving the photoresponsivity and detectivity of MoS2-based devices. To elucidate the underlying mechanisms contributing to this enhancement, power- and wavelength-dependent photoresponses, along with material characterizations based on spectroscopic, chemical, morphological measurements, and analyses, are discussed.
CitationPak, Y., Mitra, S., Alaal, N., Xin, B., Lopatin, S., Almalawi, D., … Roqan, I. S. (2020). Dark-current reduction accompanied photocurrent enhancement in p-type MnO quantum-dot decorated n-type 2D-MoS2-based photodetector. Applied Physics Letters, 116(11), 112102. doi:10.1063/1.5143578
JournalApplied Physics Letters