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dc.contributor.authorCadiau, Amandine
dc.contributor.authorXie, Lilia S.
dc.contributor.authorKolobov, Nikita
dc.contributor.authorShkurenko, Aleksander
dc.contributor.authorQureshi, Muhammad
dc.contributor.authorTchalala, Mohammed
dc.contributor.authorPark, Sarah S.
dc.contributor.authorBavykina, Anastasiya
dc.contributor.authorEddaoudi, Mohamed
dc.contributor.authorDincǎ, Mircea
dc.contributor.authorHendon, Christopher H.
dc.contributor.authorGascon, Jorge
dc.date.accessioned2020-02-04T07:25:45Z
dc.date.available2020-02-04T07:25:45Z
dc.date.issued2019-12-18
dc.date.submitted2019-06-24
dc.identifier.citationCadiau, A., Xie, L. S., Kolobov, N., Shkurenko, A., Qureshi, M., Tchalala, M. R., … Gascon, J. (2019). Toward New 2D Zirconium-Based Metal–Organic Frameworks: Synthesis, Structures, and Electronic Properties. Chemistry of Materials, 32(1), 97–104. doi:10.1021/acs.chemmater.9b02462
dc.identifier.doi10.1021/acs.chemmater.9b02462
dc.identifier.urihttp://hdl.handle.net/10754/661365
dc.description.abstractNowadays, zirconium metal-organic frameworks attract more attention because of their robustness and their easier predictability in terms of topology. Herein, we have been able to control synthetic parameters in order to construct two new 2D MOFs with the same sql topology. Both materials, ACM-10 and ACM-11, have been characterized by single-crystal X-ray diffraction, thermogravimetric analysis, and UV-vis spectroscopy. Their textural, electrochemical, and conductivity properties are presented along with the opportunities that these new topologically interesting scaffolds offer for the design of new structures.
dc.description.sponsorshipThe work at MIT was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences (DESC0018235). L.S.X. and S.S.P. thank the National Science Foundation for support through the Graduate Research Fellowship Program (1122374). A.C. thanks the program P.I.A “MOPGA” (APPAT) for funding. This work used the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by the National Science Foundation grant number ACI-1548562, and the PICS machine, Coeus, which is supported by the NSF (DMS1624776). The KAUST Office of Sponsored Research is gratefully acknowledged for funding through the 2019 CRG program.
dc.publisherAmerican Chemical Society (ACS)
dc.relation.urlhttps://pubs.acs.org/doi/10.1021/acs.chemmater.9b02462
dc.rightsThis document is the Accepted Manuscript version of a Published Work that appeared in final form in Chemistry of Materials, copyright © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see https://pubs.acs.org/doi/10.1021/acs.chemmater.9b02462.
dc.titleToward New 2D Zirconium-Based Metal–Organic Frameworks: Synthesis, Structures, and Electronic Properties
dc.typeArticle
dc.contributor.departmentAdvanced Membranes and Porous Materials Research Center
dc.contributor.departmentChemical Science Program
dc.contributor.departmentFunctional Materials Design, Discovery and Development (FMD3)
dc.contributor.departmentKAUST Catalysis Center (KCC)
dc.contributor.departmentPhysical Science and Engineering (PSE) Division
dc.identifier.journalChemistry of Materials
dc.rights.embargodate2020-12-18
dc.eprint.versionPost-print
dc.contributor.institutionDepartment of Chemistry, Massachusetts Institute of Technology, 77 Massachusetts Avenue, Cambridge, Massachusetts 02139, United States
dc.contributor.institutionMaterials Science Institute, Department of Chemistry and Biochemistry, University of Oregon, Eugene, Oregon 97403, United States
kaust.personCadiau, Amandine
kaust.personKolobov, Nikita
kaust.personShkurenko, Aleksander
kaust.personQureshi, Muhammad
kaust.personTchalala, Mohammed
kaust.personBavykina, Anastasiya
kaust.personEddaoudi, Mohamed
dc.date.accepted2019-12-17
dc.relation.issupplementedbyDOI:10.5517/ccdc.csd.cc223pws
dc.relation.issupplementedbyDOI:10.5517/ccdc.csd.cc223r65
refterms.dateFOA2020-02-04T10:46:15Z
display.relations<b> Is Supplemented By:</b> <br/> <ul> <li><i>[Dataset]</i> <br/> . DOI: <a href="https://doi.org/10.5517/ccdc.csd.cc223pws">10.5517/ccdc.csd.cc223pws</a> HANDLE: <a href="http://hdl.handle.net/10754/664843">10754/664843</a></li></ul><b> Is Supplemented By:</b> <br/> <ul> <li><i>[Dataset]</i> <br/> . DOI: <a href="https://doi.org/10.5517/ccdc.csd.cc223r65">10.5517/ccdc.csd.cc223r65</a> HANDLE: <a href="http://hdl.handle.net/10754/664844">10754/664844</a></li></ul>
kaust.acknowledged.supportUnitKAUST Office of Sponsored Research
dc.date.published-online2019-12-18
dc.date.published-print2020-01-14


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