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    Low-Temperature Cross-Linking Benzocyclobutene Based Polymer Dielectric for Organic Thin Film Transistors on Plastic Substrates.

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    Type
    Article
    Authors
    Hallani, Rawad K
    Moser, Maximilian
    Bristow, Helen
    Jenart, Maud V C
    Faber, Hendrik cc
    Neophytou, Marios cc
    Yarali, Emre cc
    Paterson, Alexandra F
    Anthopoulos, Thomas D. cc
    McCulloch, Iain cc
    KAUST Department
    Chemical Science Program
    KAUST Solar Center (KSC)
    Material Science and Engineering Program
    Physical Science and Engineering (PSE) Division
    Date
    2019-11-29
    Online Publication Date
    2019-11-29
    Print Publication Date
    2020-01-03
    Embargo End Date
    2020-11-30
    Permanent link to this record
    http://hdl.handle.net/10754/660595
    
    Metadata
    Show full item record
    Abstract
    The synthesis of a new benzocyclobutene based polymer, PSBBB, designed as a dielectric material for use in organic thin film transistors was reported. Compared to conventional benzocyclobutene-based materials, the introduction of a butoxide substituent at the 7-position of the benzocyclobutene pendant unit on the polymer allowed PSBBB to be cross-linked at temperatures of 120 °C, thus rendering it compatible with the processing requirements of flexible plastic substrates. The cross-linking behavior of PSBBB was investigated by Fourier transform infrared spectroscopy and differential scanning calorimetry, demonstrating cross-linking of the polymer after curing at 120 °C. Bottom-gate bottom-contact organic thin film transistors were fabricated using PSBBB as dielectric, affording a performance comparable to that of other dielectric polymeric materials.
    Citation
    Hallani, R. K., Moser, M., Bristow, H., Jenart, M. V. C., Faber, H., Neophytou, M., … McCulloch, I. (2019). A low temperature crosslinking benzocyclobutene based polymer dielectric for organic thin film transistors on plastic substrates. The Journal of Organic Chemistry. doi:10.1021/acs.joc.9b02981
    Sponsors
    The research reported in this publication was supported by funding from King Abdullah University of Science and Technology (KAUST).
    Publisher
    American Chemical Society (ACS)
    Journal
    The Journal of organic chemistry
    DOI
    10.1021/acs.joc.9b02981
    Additional Links
    https://pubs.acs.org/doi/10.1021/acs.joc.9b02981
    ae974a485f413a2113503eed53cd6c53
    10.1021/acs.joc.9b02981
    Scopus Count
    Collections
    Articles; Physical Science and Engineering (PSE) Division; Chemical Science Program; Material Science and Engineering Program; KAUST Solar Center (KSC)

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