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    Processing-Performance Evolution of Perovskite Solar Cells: From Large Grain Polycrystalline Films to Single Crystals

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    Name:
    Processing-Performance Evolution of Perovskite Solar Cells.pdf
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    1.404Mb
    Format:
    PDF
    Description:
    Accepted manuscript
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    Type
    Article
    Authors
    Haque, Mohammed
    Troughton, Joel
    Baran, Derya cc
    KAUST Department
    KAUST Solar Center (KSC)
    Material Science and Engineering Program
    Physical Science and Engineering (PSE) Division
    KAUST Grant Number
    OSR-CRG2018-3737
    Date
    2019-11-26
    Online Publication Date
    2019-11-26
    Print Publication Date
    2020-04
    Embargo End Date
    2020-11-26
    Permanent link to this record
    http://hdl.handle.net/10754/660462
    
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    Abstract
    Solution-processable halide perovskites have emerged as strong contenders for next-generation solar cells owing to their favorable optoelectronic properties. To maintain the efficiency momentum of perovskite solar cells (PSCs), development of advanced processing techniques, particularly for the perovskite layer, is imperative. There is a close correlation between the quality of the perovskite layer and its photophysical properties: Highly crystalline large grains with uniform morphology of the perovskite layer and their interface with charge transporters are crucial for achieving high performance. Significant efforts have been dedicated to achieve perovskite films with large grains reaching the millimeter-scale for high-efficiency PSCs. Recent work showcases a transition from large grain polycrystalline to single-crystalline (SC) PSCs made possible by the facile growth of perovskite single crystals. In this review, the recent progress of the large grain polycrystalline PSCs and grain boundary-free SC-PSCs is reported, particularly focusing on the recent approach of depositing large-grained perovskite layers and single crystal growth technique, that have been adopted for fabrication of efficient PSCs. In addition, prospects of SC-PSCs and their further development in terms of efficiency, device design, scalability, and stability are discussed.
    Citation
    Haque, M. A., Troughton, J., & Baran, D. (2019). Processing-Performance Evolution of Perovskite Solar Cells: From Large Grain Polycrystalline Films to Single Crystals. Advanced Energy Materials, 1902762. doi:10.1002/aenm.201902762
    Sponsors
    This publication is based upon work supported by the King Abdullah University of Science and Technology (KAUST) Office of Sponsored Research (OSR) under Award No. OSR-CRG2018-3737.
    Publisher
    Wiley
    Journal
    Advanced Energy Materials
    DOI
    10.1002/aenm.201902762
    Additional Links
    https://onlinelibrary.wiley.com/doi/abs/10.1002/aenm.201902762
    ae974a485f413a2113503eed53cd6c53
    10.1002/aenm.201902762
    Scopus Count
    Collections
    Articles; Physical Science and Engineering (PSE) Division; Material Science and Engineering Program; KAUST Solar Center (KSC)

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