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    Hydrodeoxygenation of raw bio-oil towards platform chemicals over FeMoP/zeolite catalysts

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    Type
    Article
    Authors
    Hita, Idoia
    Cordero-Lanzac, Tomás cc
    Bonura, Giuseppe cc
    Cannilla, Catia
    Arandes, José M.
    Frusteri, Francesco cc
    Bilbao, Javier
    KAUST Department
    Multiscale Reaction Engineering, KAUST Catalysis Center (KCC), King Abdullah University of Science and Technology (KAUST), Thuwal, 23955-6900, Saudi Arabia
    Date
    2019-08-09
    Online Publication Date
    2019-08-09
    Print Publication Date
    2019-08
    Permanent link to this record
    http://hdl.handle.net/10754/656824
    
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    Abstract
    The hydrodeoxygenation of raw bio-oil was investigated in a continuous fixed bed reactor over a series of FeMoP/zeolite catalysts, pursuing a maximized and stable production of phenolics and aromatics. After 5 h of reaction, the catalysts reach a pseudosteady activity state. The FeMoP/HZSM-5 catalyst yields the highest amount of carbon products (53.5 wt%) with the highest selectivity towards aromatics (13.6 wt%, dry basis) and phenolics (12.2 wt%), due to the synergy between the weak acidity of the FeMoP and the mild acidity of the HZSM-5 zeolite, which minimizes dehydration and gasification. The MFI framework allows the sweeping of coke precursors.
    Citation
    Hita, I., Cordero-Lanzac, T., Bonura, G., Cannilla, C., Arandes, J. M., Frusteri, F., & Bilbao, J. (2019). Hydrodeoxygenation of raw bio-oil towards platform chemicals over FeMoP/zeolite catalysts. Journal of Industrial and Engineering Chemistry, 80, 392–400. doi:10.1016/j.jiec.2019.08.019
    Sponsors
    This work was carried out with the support of the Ministry of Economy and Competitiveness of the Spanish Government, some cofounded with ERDF funds (CTQ2015-67425-R), the Basque Government (IT1218-19) and the European Commission (Horizon H2020-MSCA RISE-2018, Contract No. 823745). Dr. Idoia Hita is grateful for her postdoctoral grant awarded by the Department of Education, University and Research of the Basque Government (POS_2015_1_0035). Authors thank Dr. Enrico Catizzone from UniCAL (Cosenza, Italy) for ICP-MS measurements.
    Publisher
    Elsevier BV
    Journal
    Journal of Industrial and Engineering Chemistry
    DOI
    10.1016/j.jiec.2019.08.019
    Additional Links
    https://linkinghub.elsevier.com/retrieve/pii/S1226086X19304228
    ae974a485f413a2113503eed53cd6c53
    10.1016/j.jiec.2019.08.019
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