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    Magnesium-Catalyzed Hydroboration of Terminal and Internal Alkynes

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    Type
    Article
    Authors
    Magre, Marc
    Maity, Bholanath cc
    Falconnet, Alban
    Cavallo, Luigi cc
    Rueping, Magnus cc
    KAUST Department
    Chemical Science Program
    KAUST Catalysis Center (KCC)
    Physical Science and Engineering (PSE) Division
    Date
    2019-04-12
    Online Publication Date
    2019-04-12
    Print Publication Date
    2019-05-20
    Permanent link to this record
    http://hdl.handle.net/10754/631875
    
    Metadata
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    Abstract
    A magnesium-catalyzed hydroboration of alkynes providing good yields and selectivities for a wide range of terminal and symmetrical and unsymmetrical internal alkynes has been developed. The compatibility with many functional groups makes this magnesium catalyzed procedure attractive for late stage functionalization. Experimental mechanistic investigations and DFT calculations reveal insights into the reaction mechanism of the magnesium catalyzed protocol.
    Citation
    Magre M, Maity B, Falconnet A, Cavallo L, Rueping M (2019) Magnesium-Catalyzed Hydroboration of Terminal and Internal Alkynes. Angewandte Chemie International Edition. Available: http://dx.doi.org/10.1002/anie.201902188.
    Sponsors
    B.M. and L.C. acknowledge King Abdullah University of Science and Technology (KAUST) for computational resources of the supercomputer Shaheen II.
    Publisher
    Wiley
    Journal
    Angewandte Chemie
    DOI
    10.1002/anie.201902188
    10.1002/ange.201902188
    Additional Links
    https://onlinelibrary.wiley.com/doi/full/10.1002/anie.201902188
    ae974a485f413a2113503eed53cd6c53
    10.1002/anie.201902188
    Scopus Count
    Collections
    Articles; Physical Science and Engineering (PSE) Division; Chemical Science Program; KAUST Catalysis Center (KCC)

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