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    Dehydrogenative Aromatization and Sulfonylation of Pyrrolidines: Orthogonal Reactivity in Photoredox Catalysis

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    Type
    Article
    Authors
    Muralirajan, Krishnamoorthy
    Kancherla, Rajesh
    Rueping, Magnus cc
    KAUST Department
    Chemical Science Program
    KAUST Catalysis Center (KCC)
    Physical Science and Engineering (PSE) Division
    Date
    2018-10-11
    Online Publication Date
    2018-10-11
    Print Publication Date
    2018-11-05
    Permanent link to this record
    http://hdl.handle.net/10754/630581
    
    Metadata
    Show full item record
    Abstract
    Oxidative dehydrogenative aromatization and selective sulfonylation reactions of N-heterocycles under visible-light photoredox catalysis were established. The mild reaction conditions make this approach an appealing and versatile strategy to functionalize/oxidize pyrrolidines whereby arylsulfonyl chlorides were identified to be both catalyst regeneration and sulfonylation reagents.
    Citation
    Muralirajan K, Kancherla R, Rueping M (2018) Dehydrogenative Aromatization and Sulfonylation of Pyrrolidines: Orthogonal Reactivity in Photoredox Catalysis. Angewandte Chemie International Edition 57: 14787–14791. Available: http://dx.doi.org/10.1002/anie.201808427.
    Sponsors
    The authors acknowledge KAUST for financial support. The research leading to these results has received funding from the European Research Council under the European Union's Seventh Framework Programme (FP/2007-2013)/ERC grant agreement number 617044 (SunCatChem).
    Publisher
    Wiley
    Journal
    Angewandte Chemie
    DOI
    10.1002/anie.201808427
    10.1002/ange.201808427
    Additional Links
    https://onlinelibrary.wiley.com/doi/full/10.1002/anie.201808427
    ae974a485f413a2113503eed53cd6c53
    10.1002/anie.201808427
    Scopus Count
    Collections
    Articles; Physical Science and Engineering (PSE) Division; Chemical Science Program; KAUST Catalysis Center (KCC)

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