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dc.contributor.authorWang, Yu
dc.contributor.authorPan, Ying
dc.contributor.authorZhu, Liangkui
dc.contributor.authorGuo, Ningning
dc.contributor.authorWang, Runwei
dc.contributor.authorZhang, Zongtao
dc.contributor.authorQiu, Shilun
dc.date.accessioned2018-11-11T09:04:29Z
dc.date.available2018-11-11T09:04:29Z
dc.date.issued2018-10-16
dc.identifier.citationWang Y, Pan Y, Zhu L, Guo N, Wang R, et al. (2019) Structure regulation of amino acids derived nitrogen doped porous carbon nanosheet through facile solid state assembly method. Microporous and Mesoporous Materials 277: 36–44. Available: http://dx.doi.org/10.1016/j.micromeso.2018.10.011.
dc.identifier.issn1387-1811
dc.identifier.doi10.1016/j.micromeso.2018.10.011
dc.identifier.urihttp://hdl.handle.net/10754/629812
dc.description.abstractCarbon nanosheets are widely used in electrocatalysis. Structure control is a great challenge in preparation of carbon materials. Here, a facial solid state assembly method is applied to prepare carbon nanosheets. By choosing amino acids as precursors, structure regulation of carbon nanosheets could be realized via switching the side chains of organic linkers, showing structure evolution from dense monolithic to porous nanosheets. Graphene-like carbon nanosheet constructed foam superstructure was also obtained. Owing to high porosity (BET surface area 1680 m2 g−1 with hierarchical pore structure) and nitrogen (8.23 wt%) modified graphitic frameworks, glutamic acid derived nitrogen doped porous carbon nanosheet superstructure showed high ORR activity (onset potential 0.9 V vs. RHE).
dc.description.sponsorshipThis work was financially supported by the National Natural Science Foundation of China (21390394, 21771082 and 21771081), National Basic Research Program of China (2012CB821700 and 2011CB808703), NSFC (21261130584 and 91022030), “111” project (B07016), Award Project of KAUST (CRG-1-2012-LAI-009) and Ministry of Education, Science and Technology Development Center Project (20120061130012).
dc.publisherElsevier BV
dc.subjectCarbon nanosheet
dc.subjectAmino acid
dc.subjectStructure regulation
dc.subjectSolvent free
dc.subjectOxygen reduction reaction
dc.titleStructure regulation of amino acids derived nitrogen doped porous carbon nanosheet through facile solid state assembly method
dc.typeArticle
dc.identifier.journalMicroporous and Mesoporous Materials
dc.contributor.institutionState Key Laboratory of Inorganic Synthesis and Preparative Chemistry, College of Chemistry, Jilin University, 2699 Qianjin Street, Changchun, PR China
kaust.grant.numberCRG-1-2012-LAI-009
dc.date.published-online2018-10-16
dc.date.published-print2019-03


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