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    Structure regulation of amino acids derived nitrogen doped porous carbon nanosheet through facile solid state assembly method

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    Type
    Article
    Authors
    Wang, Yu
    Pan, Ying
    Zhu, Liangkui
    Guo, Ningning
    Wang, Runwei cc
    Zhang, Zongtao
    Qiu, Shilun
    KAUST Grant Number
    CRG-1-2012-LAI-009
    Date
    2018-10-16
    Online Publication Date
    2018-10-16
    Print Publication Date
    2019-03
    Permanent link to this record
    http://hdl.handle.net/10754/629812
    
    Metadata
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    Abstract
    Carbon nanosheets are widely used in electrocatalysis. Structure control is a great challenge in preparation of carbon materials. Here, a facial solid state assembly method is applied to prepare carbon nanosheets. By choosing amino acids as precursors, structure regulation of carbon nanosheets could be realized via switching the side chains of organic linkers, showing structure evolution from dense monolithic to porous nanosheets. Graphene-like carbon nanosheet constructed foam superstructure was also obtained. Owing to high porosity (BET surface area 1680 m2 g−1 with hierarchical pore structure) and nitrogen (8.23 wt%) modified graphitic frameworks, glutamic acid derived nitrogen doped porous carbon nanosheet superstructure showed high ORR activity (onset potential 0.9 V vs. RHE).
    Citation
    Wang Y, Pan Y, Zhu L, Guo N, Wang R, et al. (2019) Structure regulation of amino acids derived nitrogen doped porous carbon nanosheet through facile solid state assembly method. Microporous and Mesoporous Materials 277: 36–44. Available: http://dx.doi.org/10.1016/j.micromeso.2018.10.011.
    Sponsors
    This work was financially supported by the National Natural Science Foundation of China (21390394, 21771082 and 21771081), National Basic Research Program of China (2012CB821700 and 2011CB808703), NSFC (21261130584 and 91022030), “111” project (B07016), Award Project of KAUST (CRG-1-2012-LAI-009) and Ministry of Education, Science and Technology Development Center Project (20120061130012).
    Publisher
    Elsevier BV
    Journal
    Microporous and Mesoporous Materials
    DOI
    10.1016/j.micromeso.2018.10.011
    ae974a485f413a2113503eed53cd6c53
    10.1016/j.micromeso.2018.10.011
    Scopus Count
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