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    Diverse catalytic reactivity of a dearomatized PN3P*-nickel hydride pincer complex towards CO2 reduction

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    Type
    Article
    Authors
    Huang, Kuo-Wei cc
    Li, Huaifeng cc
    Goncalves, Theo
    Zhao, Qianyi
    Gong, Dirong
    Lai, Zhiping cc
    Wang, Zhi-Xiang
    Zheng, Junrong
    KAUST Department
    Advanced Membranes and Porous Materials Research Center
    Chemical Engineering Program
    Chemical Science Program
    Homogeneous Catalysis Laboratory (HCL)
    KAUST Catalysis Center (KCC)
    Physical Science and Engineering (PSE) Division
    Date
    2018
    Permanent link to this record
    http://hdl.handle.net/10754/628474
    
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    Abstract
    A dearomatized PN3P*-nickel hydride complex has been prepared by oxidative addition process. The first nickel-catalyzed hydrosilylation of CO2 to methanol has been achieved, with unprecedented turnover numbers. Selectvie methylation and formylation of amines with CO2 were demonstrated by such PN3P*-nickel hydride complex, highlighting its versatile functions in CO2 reduction.
    Citation
    Li H, Gonçalves TP, Zhao Q, Gong D, Lai Z, et al. (2018) Diverse catalytic reactivity of a dearomatized PN3P*–nickel hydride pincer complex towards CO2 reduction. Chemical Communications. Available: http://dx.doi.org/10.1039/c8cc05948a.
    Publisher
    Royal Society of Chemistry (RSC)
    Journal
    Chemical Communications
    DOI
    10.1039/c8cc05948a
    Additional Links
    http://pubs.rsc.org/en/Content/ArticleLanding/2018/CC/C8CC05948A#!divAbstract
    Relations
    Is Supplemented By:
    • [Dataset]
      . DOI: 10.5517/ccdc.csd.cc1pqst0 HANDLE: 10754/664147
    Is Supplemented By:
    • [Dataset]
      . DOI: 10.5517/ccdc.csd.cc1nc4rx HANDLE: 10754/664148
    Is Supplemented By:
    • [Dataset]
      . DOI: 10.5517/ccdc.csd.cc1mjtnm HANDLE: 10754/664149
    ae974a485f413a2113503eed53cd6c53
    10.1039/c8cc05948a
    Scopus Count
    Collections
    Articles; Advanced Membranes and Porous Materials Research Center; Physical Science and Engineering (PSE) Division; Chemical Science Program; Chemical Engineering Program; KAUST Catalysis Center (KCC)

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