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    Reversible Switching and Recycling of Adaptable Organic Microgel Catalysts (Microgelzymes) for Asymmetric Organocatalytic Desymmetrization

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    Type
    Article
    Authors
    Borrmann, Ruediger
    Palchyk, Volodymyr
    Pich, Andrij
    Rueping, Magnus
    KAUST Department
    KAUST Catalysis Center (KCC)
    Date
    2018-08
    Online Publication Date
    2018-08
    Print Publication Date
    2018-09-07
    Permanent link to this record
    http://hdl.handle.net/10754/628294
    
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    Abstract
    Adaptable enzyme-mimetic catalysts based on temperature-responsive polymer microgels (microgelzymes) have been developed. By a simple change in the temperature, a microgel catalyst can be reversibly switched into its soluble or precipitated form, thus combining the advantages of homogeneous and heterogeneous catalysis. The responsive microgel reactors show high reactivity and selectivity, as well as good recycling properties in the alcoholysis of cis-tetrahydrophthalic anhydride.
    Citation
    Borrmann R, Palchyk V, Pich A, Rueping M (2018) Reversible Switching and Recycling of Adaptable Organic Microgel Catalysts (Microgelzymes) for Asymmetric Organocatalytic Desymmetrization. ACS Catalysis: 7991–7996. Available: http://dx.doi.org/10.1021/acscatal.8b01408.
    Sponsors
    We thank the BMBF (Project UGR203118812), German Research Foundation (DFG) SFB 985 “Functional Microgels and Microgel Systems” (A.P.), and the Volkswagen Foundation (A.P.) for financial support.
    Publisher
    American Chemical Society (ACS)
    Journal
    ACS Catalysis
    DOI
    10.1021/acscatal.8b01408
    Additional Links
    https://pubs.acs.org/doi/10.1021/acscatal.8b01408
    ae974a485f413a2113503eed53cd6c53
    10.1021/acscatal.8b01408
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