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    Metal-Organic-Framework-Mediated Nitrogen-Doped Carbon for CO2 Electrochemical Reduction

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    Type
    Article
    Authors
    Wang, Riming
    Sun, Xiaohui
    Ould-Chikh, Samy cc
    Osadchii, Dmitrii
    Bai, Fan
    Kapteijn, Freek cc
    Gascon, Jorge cc
    KAUST Department
    Chemical Engineering Program
    KAUST Catalysis Center (KCC)
    Physical Science and Engineering (PSE) Division
    Date
    2018-04-11
    Online Publication Date
    2018-04-11
    Print Publication Date
    2018-05-02
    Permanent link to this record
    http://hdl.handle.net/10754/627587
    
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    Abstract
    A nitrogen-doped carbon was synthesized through the pyrolysis of the well-known metal-organic framework ZIF-8, followed by a subsequent acid treatment, and has been applied as a catalyst in the electrochemical reduction of carbon dioxide. The resulting electrode shows Faradaic efficiencies to carbon monoxide as high as ∼78%, with hydrogen being the only byproduct. The pyrolysis temperature determines the amount and the accessibility of N species in the carbon electrode, in which pyridinic-N and quaternary-N species play key roles in the selective formation of carbon monoxide.
    Citation
    Wang R, Sun X, Ould-Chikh S, Osadchii D, Bai F, et al. (2018) Metal-Organic-Framework-Mediated Nitrogen-Doped Carbon for CO2 Electrochemical Reduction. ACS Applied Materials & Interfaces. Available: http://dx.doi.org/10.1021/acsami.8b02226.
    Sponsors
    The authors would like to thank the China Scholarship Council (CSC) for financial support.
    Publisher
    American Chemical Society (ACS)
    Journal
    ACS Applied Materials & Interfaces
    DOI
    10.1021/acsami.8b02226
    PubMed ID
    29638117
    Additional Links
    https://pubs.acs.org/doi/10.1021/acsami.8b02226
    ae974a485f413a2113503eed53cd6c53
    10.1021/acsami.8b02226
    Scopus Count
    Collections
    Articles; Physical Science and Engineering (PSE) Division; Chemical Engineering Program; KAUST Catalysis Center (KCC)

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