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dc.contributor.authorHwang, Seungtaik
dc.contributor.authorSemino, Rocio
dc.contributor.authorSeoane, Beatriz
dc.contributor.authorZahan, Marufa
dc.contributor.authorChmelik, Christian
dc.contributor.authorValiullin, Rustem
dc.contributor.authorBertmer, Marko
dc.contributor.authorHaase, Jürgen
dc.contributor.authorKapteijn, Freek
dc.contributor.authorGascon, Jorge
dc.contributor.authorMaurin, Guillaume
dc.contributor.authorKärger, Jörg
dc.date.accessioned2018-02-27T09:00:12Z
dc.date.available2018-02-27T09:00:12Z
dc.date.issued2018-03-25
dc.identifier.citationHwang S, Semino R, Seoane B, Zahan M, Chmelik C, et al. (2018) Revealing Transient Concentration of CO2 in a Mixed Matrix Membrane by IR Microimaging and Molecular Modeling. Angewandte Chemie International Edition. Available: http://dx.doi.org/10.1002/anie.201713160.
dc.identifier.issn1433-7851
dc.identifier.doi10.1002/anie.201713160
dc.identifier.doi10.1002/ange.201713160
dc.identifier.urihttp://hdl.handle.net/10754/627202
dc.description.abstractThrough IR microimaging the spatially and temporally resolved development of the CO2 concentration in a ZIF-8@6FDA-DAM mixed matrix membrane was visualized during transient adsorption. By recording the evolution of the CO2 concentration, it is observed that the CO2 molecules propagate from the ZIF-8 filler, which acts as a transport
dc.description.sponsorshipThe research leading to these results has received funding from the European Community Seventh Program (FP7/2007-2013) under Grant 608490 (project M4CO2). IR microimaging was ensured by German Science Foundation via the grants HA 1893/17-1 and KA 953/35-1. G.M. thanks Institut Universitaire de France for its support. The authors thank J. Caro (Hannover) for stimulating discussions and synthesizing the large ZIF-8 crystals.
dc.publisherWiley
dc.relation.urlhttp://onlinelibrary.wiley.com/doi/10.1002/anie.201713160/abstract
dc.rightsThis is the peer reviewed version of the following article: Revealing Transient Concentration of CO2 in a Mixed Matrix Membrane by IR Microimaging and Molecular Modeling, which has been published in final form at http://doi.org/10.1002/anie.201713160. This article may be used for non-commercial purposes in accordance With Wiley Terms and Conditions for self-archiving.
dc.subjectMolecular modeling
dc.subjectIR spectroscopy
dc.subjectadsorption
dc.subjectInterfaces
dc.subjectMixed Matrix Membrane
dc.titleRevealing Transient Concentration of CO2 in a Mixed Matrix Membrane by IR Microimaging and Molecular Modeling
dc.typeArticle
dc.contributor.departmentChemical Engineering Program
dc.contributor.departmentKAUST Catalysis Center (KCC)
dc.contributor.departmentPhysical Science and Engineering (PSE) Division
dc.identifier.journalAngewandte Chemie International Edition
dc.eprint.versionPost-print
dc.contributor.institutionUniversity of Leipzig; Faculty of Physics and Earth Sciences; Linnéstrasse 5 04103 Leipzig GERMANY
dc.contributor.institutionÉcole Polytechnique Fédérale de Lausanne; Institute of Materials; Route Cantonale 1015 Lausanne SWITZERLAND
dc.contributor.institutionUtrecht University; Debye Institute for Nanomaterials Science; Universiteitsweg 99 3584 CG Utrecht NETHERLANDS
dc.contributor.institutionUniversity of Leipzig; Faculty of Physic and Earth Sciences; Linnéstrasse 5 04103 Leipzig GERMANY
dc.contributor.institutionDelft University of Technology; Catalysis Engineering, ChemE Department; Van der Maasweg 9 2629 HZ Delft NETHERLANDS
dc.contributor.institutionUniversité de Montpellier; Institut Charles Gerhardt Montpellier; Place Eugène Bataillon 34095 Montpellier FRANCE
dc.contributor.institutionUniversity of Leipzig; Department of Interface Physics; Linnéstrasse 5 04103 Leipzig GERMANY
kaust.personGascon, Jorge
refterms.dateFOA2019-02-21T00:00:00Z
dc.date.published-online2018-03-25
dc.date.published-print2018-04-23


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