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    Revealing Transient Concentration of CO2 in a Mixed Matrix Membrane by IR Microimaging and Molecular Modeling

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    Hwang_et_al-2018-Angewandte_Chemie_International_Edition.pdf
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    Type
    Article
    Authors
    Hwang, Seungtaik
    Semino, Rocio
    Seoane, Beatriz
    Zahan, Marufa
    Chmelik, Christian
    Valiullin, Rustem
    Bertmer, Marko
    Haase, Jürgen
    Kapteijn, Freek cc
    Gascon, Jorge cc
    Maurin, Guillaume cc
    Kärger, Jörg
    KAUST Department
    Chemical Engineering Program
    KAUST Catalysis Center (KCC)
    Physical Science and Engineering (PSE) Division
    Date
    2018-03-25
    Online Publication Date
    2018-03-25
    Print Publication Date
    2018-04-23
    Permanent link to this record
    http://hdl.handle.net/10754/627202
    
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    Abstract
    Through IR microimaging the spatially and temporally resolved development of the CO2 concentration in a ZIF-8@6FDA-DAM mixed matrix membrane was visualized during transient adsorption. By recording the evolution of the CO2 concentration, it is observed that the CO2 molecules propagate from the ZIF-8 filler, which acts as a transport
    Citation
    Hwang S, Semino R, Seoane B, Zahan M, Chmelik C, et al. (2018) Revealing Transient Concentration of CO2 in a Mixed Matrix Membrane by IR Microimaging and Molecular Modeling. Angewandte Chemie International Edition. Available: http://dx.doi.org/10.1002/anie.201713160.
    Sponsors
    The research leading to these results has received funding from the European Community Seventh Program (FP7/2007-2013) under Grant 608490 (project M4CO2). IR microimaging was ensured by German Science Foundation via the grants HA 1893/17-1 and KA 953/35-1. G.M. thanks Institut Universitaire de France for its support. The authors thank J. Caro (Hannover) for stimulating discussions and synthesizing the large ZIF-8 crystals.
    Publisher
    Wiley-Blackwell
    Journal
    Angewandte Chemie International Edition
    DOI
    10.1002/anie.201713160
    10.1002/ange.201713160
    Additional Links
    http://onlinelibrary.wiley.com/doi/10.1002/anie.201713160/abstract
    ae974a485f413a2113503eed53cd6c53
    10.1002/anie.201713160
    Scopus Count
    Collections
    Articles; Physical Science and Engineering (PSE) Division; Chemical Engineering Program; KAUST Catalysis Center (KCC)

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