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    Epitaxial Growth of Two-Dimensional Layered Transition-Metal Dichalcogenides: Growth Mechanism, Controllability, and Scalability

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    Type
    Article
    Authors
    Li, Henan
    Li, Ying
    Aljarb, Areej
    Shi, Yumeng
    Li, Lain-Jong cc
    KAUST Department
    KAUST Catalysis Center (KCC)
    Material Science and Engineering Program
    Physical Science and Engineering (PSE) Division
    Date
    2017-07-06
    Online Publication Date
    2017-07-06
    Print Publication Date
    2018-07-11
    Permanent link to this record
    http://hdl.handle.net/10754/625664
    
    Metadata
    Show full item record
    Abstract
    Recently there have been many research breakthroughs in two-dimensional (2D) materials including graphene, boron nitride (h-BN), black phosphors (BPs), and transition-metal dichalcogenides (TMDCs). The unique electrical, optical, and thermal properties in 2D materials are associated with their strictly defined low dimensionalities. These materials provide a wide range of basic building blocks for next-generation electronics. The chemical vapor deposition (CVD) technique has shown great promise to generate high-quality TMDC layers with scalable size, controllable thickness, and excellent electronic properties suitable for both technological applications and fundamental sciences. The capability to precisely engineer 2D materials by chemical approaches has also given rise to fascinating new physics, which could lead to exciting new applications. In this Review, we introduce the latest development of TMDC synthesis by CVD approaches and provide further insight for the controllable and reliable synthesis of atomically thin TMDCs. Understanding of the vapor-phase growth mechanism of 2D TMDCs could benefit the formation of complicated heterostructures and novel artificial 2D lattices.
    Citation
    Li H, Li Y, Aljarb A, Shi Y, Li L-J (2017) Epitaxial Growth of Two-Dimensional Layered Transition-Metal Dichalcogenides: Growth Mechanism, Controllability, and Scalability. Chemical Reviews. Available: http://dx.doi.org/10.1021/acs.chemrev.7b00212.
    Sponsors
    This work was supported by National Natural Science Foundation of China (Grant no. 51602200), Educational Commission of Guangdong Province (Grant no. 2016KZDXM008), Natural Science Foundation of SZU (Grant no. 2017011), and King Abdullah University of Science and Technology, Saudi Arabia. This work was partially supported by the Science and Technology Planning Project of Guangdong Province (Grant no. 2016B050501005), the Educational Commission of Guangdong Province (Grant no. 2016KCXTD006), and Shenzhen Peacock Plan (Grant no. KQTD2016053112042971).
    Publisher
    American Chemical Society (ACS)
    Journal
    Chemical Reviews
    DOI
    10.1021/acs.chemrev.7b00212
    PubMed ID
    28682055
    Additional Links
    http://pubs.acs.org/doi/abs/10.1021/acs.chemrev.7b00212
    ae974a485f413a2113503eed53cd6c53
    10.1021/acs.chemrev.7b00212
    Scopus Count
    Collections
    Articles; Physical Science and Engineering (PSE) Division; Material Science and Engineering Program; KAUST Catalysis Center (KCC)

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