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    Nickel-Catalyzed C–O Bond-Cleaving Alkylation of Esters: Direct Replacement of the Ester Moiety by Functionalized Alkyl Chains

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    Manuscript_revised.pdf
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    Description:
    Accepted Manuscript
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    Type
    Article
    Authors
    Liu, Xiangqian
    Jia, Jiaqi
    Rueping, Magnus cc
    KAUST Department
    Chemical Science Program
    KAUST Catalysis Center (KCC)
    Physical Science and Engineering (PSE) Division
    Date
    2017-06-07
    Online Publication Date
    2017-06-07
    Print Publication Date
    2017-07-07
    Permanent link to this record
    http://hdl.handle.net/10754/625106
    
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    Abstract
    Two efficient protocols for the nickel-catalyzed aryl–alkyl cross-coupling reactions using esters as coupling components have been established. The methods enable the selective oxidative addition of nickel to acyl C–O and aryl C–O bonds and allow the aryl–alkyl cross-coupling via decarbonylative bond cleavage or through cleavage of a C–O bond with high efficiency and good functional group compatibility. The protocols allow the streamlined, unconventional utilization of widespread ester groups and their precursors, carboxylic acids and phenols, in synthetic organic chemistry.
    Citation
    Liu X, Jia J, Rueping M (2017) Nickel-Catalyzed C–O Bond-Cleaving Alkylation of Esters: Direct Replacement of the Ester Moiety by Functionalized Alkyl Chains. ACS Catalysis 7: 4491–4496. Available: http://dx.doi.org/10.1021/acscatal.7b00941.
    Sponsors
    X.L. was supported by the China Scholarship Council.
    Publisher
    American Chemical Society (ACS)
    Journal
    ACS Catalysis
    DOI
    10.1021/acscatal.7b00941
    Additional Links
    http://pubs.acs.org/doi/full/10.1021/acscatal.7b00941
    ae974a485f413a2113503eed53cd6c53
    10.1021/acscatal.7b00941
    Scopus Count
    Collections
    Articles; Physical Science and Engineering (PSE) Division; Chemical Science Program; KAUST Catalysis Center (KCC)

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