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    An Alternating 5,5-Dimethylcyclopentadiene-based Copolymer prepared at Room Temperature for High Performance Organic Thin Film Transistors

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    Name:
    jacs2E7b03279.pdf
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    Description:
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    Type
    Article
    Authors
    Fei, Zhuping
    Chen, Lei
    Han, Yang
    Gann, Eliot
    Chesman, Anthony
    McNeill, Christopher R.
    Anthopoulos, Thomas D. cc
    Heeney, Martin
    Pietrangelo, Agostino
    KAUST Department
    KAUST Solar Center (KSC)
    Material Science and Engineering Program
    Physical Science and Engineering (PSE) Division
    Date
    2017-06-12
    Online Publication Date
    2017-06-12
    Print Publication Date
    2017-06-21
    Permanent link to this record
    http://hdl.handle.net/10754/624897
    
    Metadata
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    Abstract
    We report that the inclusion of non-aromatic 5,5-dimethylcyclopentadiene monomer into a conjugated backbone is an attractive strategy to high performance semiconducting polymers. The use of this monomer enables a room temperature Suzuki copolymerization with a diketopyrrolopyrrole comono-mer to afford a highly soluble, high molecular weight material. The resulting low band gap polymer exhibits excellent photo and thermal stability, and despite a large π-π stacking distance of 4.26 Å, it demonstrates excellent performance in thin-film transistor devices.
    Citation
    Fei Z, Chen L, Han Y, Gann E, Chesman A, et al. (2017) An Alternating 5,5-Dimethylcyclopentadiene-based Copolymer prepared at Room Temperature for High Performance Organic Thin Film Transistors. Journal of the American Chemical Society. Available: http://dx.doi.org/10.1021/jacs.7b03279.
    Sponsors
    We thank Rutgers University, the British Council (173601536) and the Australian Research Council (DP130101861) for the financial support. This work was performed in part on the SAXS/WAXS beamline at the Australian Synchrotron, Victoria, Australia.
    Publisher
    American Chemical Society (ACS)
    Journal
    Journal of the American Chemical Society
    DOI
    10.1021/jacs.7b03279
    PubMed ID
    28578574
    Additional Links
    http://pubs.acs.org/doi/abs/10.1021/jacs.7b03279
    ae974a485f413a2113503eed53cd6c53
    10.1021/jacs.7b03279
    Scopus Count
    Collections
    Articles; Physical Science and Engineering (PSE) Division; Physical Science and Engineering (PSE) Division; Material Science and Engineering Program; Material Science and Engineering Program; KAUST Solar Center (KSC); KAUST Solar Center (KSC)

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