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    Efficient Electrocatalytic Reduction of CO2 by Nitrogen-Doped Nanoporous Carbon/Carbon Nanotube Membranes - A Step Towards the Electrochemical CO2 Refinery

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    Type
    Article
    Authors
    Wang, Hong
    Jia, Jia
    Song, Pengfei
    Wang, Qiang
    Li, Debao
    Min, Shixiong cc
    Qian, Chenxi
    Wang, Lu
    Li, Young Feng
    Ma, Chun
    Wu, Tao cc
    Yuan, Jiayin
    Antonietti, Markus
    Ozin, Geoffrey A.
    KAUST Department
    Laboratory of Nano Oxides for Sustainable Energy
    Material Science and Engineering Program
    Physical Science and Engineering (PSE) Division
    Date
    2017-06-01
    Online Publication Date
    2017-06-01
    Print Publication Date
    2017-06-26
    Permanent link to this record
    http://hdl.handle.net/10754/623632
    
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    Abstract
    The search for earth abundant, efficient and stable electrocatalysts that can enable the chemical reduction of CO2 to value-added chemicals and fuels at an industrially relevant scale, is a high priority for the development of a global network of renewable energy conversion and storage systems that can meaningfully impact greenhouse gas induced climate change. Here we introduce a straightforward, low cost, scalable and technologically relevant method to manufacture an all-carbon, electroactive, nitrogen-doped nanoporous carbon-carbon nanotube composite membrane. The membrane is demonstrated to function as a binder-free, high-performance electrode for the electrocatalytic reduction of CO2 to formate. The Faradaic efficiency for the production of formate is 81%. Furthermore, the robust structural and electrochemical properties of the membrane endow it with excellent long-term stability.
    Citation
    Wang H, Jia J, Song P, Wang Q, Li D, et al. (2017) Efficient Electrocatalytic Reduction of CO2 by Nitrogen-Doped Nanoporous Carbon/Carbon Nanotube Membranes - A Step Towards the Electrochemical CO2 Refinery. Angewandte Chemie International Edition. Available: http://dx.doi.org/10.1002/anie.201703720.
    Sponsors
    G.A.O. is a Government of Canada Research Chair in Materials Chem istry and Nanochemistry. Financial support for this work was provided by the Ontario Ministry of Research Innovation (MRI); Ministry of Economic Development, Employment and Infrastructure (MEDI); Ministry of the Environment and Climate Change; Connaught Innovation Fund; Connaught Global Challenge Fund; and the Natural Sciences and Engineering Research Council of Canada (NSERC). S. M. acknowledges the financial support from the National Natural Science Foundation of China (21463001). J. Y. is grateful for financial support from the Max Planck society, Germany, Clarkson University, USA and the ERC (European Research Council) Starting Grant (project number 639720-NAPOLI).
    Publisher
    Wiley-Blackwell
    Journal
    Angewandte Chemie International Edition
    DOI
    10.1002/anie.201703720
    10.1002/ange.201703720
    arXiv
    arXiv:1905.01466
    Additional Links
    http://onlinelibrary.wiley.com/doi/10.1002/anie.201703720/abstract;jsessionid=9AC18E02CA45212A56BBE52387F9B336.f03t01
    ae974a485f413a2113503eed53cd6c53
    10.1002/anie.201703720
    Scopus Count
    Collections
    Articles; Physical Science and Engineering (PSE) Division; Material Science and Engineering Program

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