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    Cyclodextrin Films with Fast Solvent Transport and Shape-Selective Permeability

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    Name:
    Manuscript Cyclodextrin Films_Mar 16.pdf
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    730.5Kb
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    PDF
    Description:
    Accepted Manuscript
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    Type
    Article
    Authors
    Villalobos, Luis Francisco cc
    Huang, Tiefan
    Peinemann, Klaus-Viktor cc
    KAUST Department
    Advanced Membranes and Porous Materials Research Center
    Chemical Engineering Program
    Physical Science and Engineering (PSE) Division
    Date
    2017-04-24
    Online Publication Date
    2017-04-24
    Print Publication Date
    2017-07
    Permanent link to this record
    http://hdl.handle.net/10754/623312
    
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    Abstract
    This study describes the molecular-level design of a new type of filtration membrane made of crosslinked cyclodextrins-inexpensive macrocycles of glucose, shaped like hollow truncated cones. The channel-like cavities of cyclodextrins spawn numerous paths of defined aperture in the separation layer that can effectively discriminate between molecules. The transport of molecules through these membranes is highly shape-sensitive. In addition, the presence of hydrophobic (cavity) and hydrophilic (ester-crosslinked outer part) domains in these films results in high permeances for both polar and nonpolar solvents.
    Citation
    Villalobos LF, Huang T, Peinemann K-V (2017) Cyclodextrin Films with Fast Solvent Transport and Shape-Selective Permeability. Advanced Materials: 1606641. Available: http://dx.doi.org/10.1002/adma.201606641.
    Sponsors
    This research was supported by King Abdullah University of Science and Technology (KAUST). The authors are grateful to Kexin Yao for assisting with the CO2 adsorption experiments and to Mohamed Nejib Hedhili for performing the XPS analysis. The authors thank Rachid Sougrat, Stefan Chisca, Mahendra Kumar, Rahul Shevate, and Federico Pacheco for discussions.
    Publisher
    Wiley
    Journal
    Advanced Materials
    DOI
    10.1002/adma.201606641
    10.1002/adma.201770187
    Additional Links
    http://onlinelibrary.wiley.com/doi/10.1002/adma.201606641/full
    ae974a485f413a2113503eed53cd6c53
    10.1002/adma.201606641
    Scopus Count
    Collections
    Articles; Advanced Membranes and Porous Materials Research Center; Physical Science and Engineering (PSE) Division; Chemical Engineering Program

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