Show simple item record

dc.contributor.authorMin, Shixiong
dc.contributor.authorYang, Xiulin
dc.contributor.authorLu, Ang-Yu
dc.contributor.authorTseng, Chien-Chih
dc.contributor.authorHedhili, Mohamed N.
dc.contributor.authorLai, Zhiping
dc.contributor.authorLi, Lain-Jong
dc.contributor.authorHuang, Kuo-Wei
dc.date.accessioned2017-04-10T07:49:52Z
dc.date.available2017-04-10T07:49:52Z
dc.date.issued2017-03-21
dc.identifier.citationMin S, Yang X, Lu A-Y, Tseng C-C, Hedhili MN, et al. (2017) Surface-reconstructed Cu electrode via a facile electrochemical anodization-reduction process for low overpotential CO 2 reduction. Journal of Saudi Chemical Society. Available: http://dx.doi.org/10.1016/j.jscs.2017.03.003.
dc.identifier.issn1319-6103
dc.identifier.doi10.1016/j.jscs.2017.03.003
dc.identifier.urihttp://hdl.handle.net/10754/623111
dc.description.abstractA high-surface-area Cu electrode, fabricated by a simple electrochemical anodization-reduction method, exhibits high activity and selectivity for CO2 reduction at low overpotential in 0.1 M KHCO3 solution. A faradaic efficiency of 37% for HCOOH and 27% for CO production was achieved with the current density of 1.5 mA cm-2 at −0.64 V vs. RHE, much higher than that of polycrystalline Cu. The enhanced catalytic performance is a result of the formation of the high electrochemical active surface area and high density of preferred low-index facets.
dc.description.sponsorshipThis work was supported by the King Abdullah University of Science and Technology (KAUST) and the National Natural Science Foundation of China (grant no. 21463001).
dc.publisherElsevier BV
dc.relation.urlhttp://www.sciencedirect.com/science/article/pii/S1319610317300388
dc.rights© 2017. This manuscript version is made available under the CC-BY-NC-ND 4.0 license http://creativecommons.org/licenses/by-nc-nd/4.0/
dc.rights.urihttp://creativecommons.org/licenses/by-nc-nd/4.0/
dc.subjectCO2 reduction
dc.subjectCu electrode
dc.subjectHigh-surface-area
dc.subjectHigh selectivity
dc.titleSurface-reconstructed Cu Electrode via a Facile Electrochemical Anodization-Reduction Process for Low Overpotential CO 2 reduction
dc.typeArticle
dc.contributor.departmentAdvanced Membranes and Porous Materials Research Center
dc.contributor.departmentChemical Engineering Program
dc.contributor.departmentChemical Science Program
dc.contributor.departmentHomogeneous Catalysis Laboratory (HCL)
dc.contributor.departmentKAUST Catalysis Center (KCC)
dc.contributor.departmentMaterial Science and Engineering Program
dc.contributor.departmentPhysical Science and Engineering (PSE) Division
dc.contributor.departmentSurface Science
dc.identifier.journalJournal of Saudi Chemical Society
dc.eprint.versionPost-print
dc.contributor.institutionSchool of Chemistry and Chemical Engineering, Beifang University of Nationalities, Yinchuan, 750021, China
kaust.personMin, Shixiong
kaust.personYang, Xiulin
kaust.personLu, Ang-Yu
kaust.personTseng, Chien-Chih
kaust.personHedhili, Mohamed N.
kaust.personLai, Zhiping
kaust.personLi, Lain-Jong
kaust.personHuang, Kuo-Wei
refterms.dateFOA2018-06-13T21:52:26Z
dc.date.published-online2017-03-21
dc.date.published-print2017-09


Files in this item

Thumbnail
Name:
1-s2.0-S1319610317300388-main.pdf
Size:
1.390Mb
Format:
PDF
Description:
Accepted Manuscript

This item appears in the following Collection(s)

Show simple item record

© 2017. This manuscript version is made available under the CC-BY-NC-ND 4.0 license http://creativecommons.org/licenses/by-nc-nd/4.0/
Except where otherwise noted, this item's license is described as © 2017. This manuscript version is made available under the CC-BY-NC-ND 4.0 license http://creativecommons.org/licenses/by-nc-nd/4.0/