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    “Self-Peel-Off” Transfer Produces Ultrathin Polyvinylidene-Fluoride-Based Flexible Nanodevices

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    Type
    Article
    Authors
    Tai, Yanlong cc
    Lubineau, Gilles cc
    KAUST Department
    Composite and Heterogeneous Material Analysis and Simulation Laboratory (COHMAS)
    Mechanical Engineering Program
    Physical Science and Engineering (PSE) Division
    Date
    2017-02-23
    Online Publication Date
    2017-02-23
    Print Publication Date
    2017-04
    Permanent link to this record
    http://hdl.handle.net/10754/622972
    
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    Abstract
    Here, a new strategy, self-peel-off transfer, for the preparation of ultrathin flexible nanodevices made from polyvinylidene-fluoride (PVDF) is reported. In this process, a functional pattern of nanoparticles is transferred via peeling from a temporary substrate to the final PVDF film. This peeling process takes advantage of the differences in the work of adhesion between the various layers (the PVDF layer, the nanoparticle-pattern layer and the substrate layer) and of the high stresses generated by the differential thermal expansion of the layers. The work of adhesion is mainly guided by the basic physical/chemical properties of these layers and is highly sensitive to variations in temperature and moisture in the environment. The peeling technique is tested on a variety of PVDF-based functional films using gold/palladium nanoparticles, carbon nanotubes, graphene oxide, and lithium iron phosphate. Several PVDF-based flexible nanodevices are prepared, including a single-sided wireless flexible humidity sensor in which PVDF is used as the substrate and a double-sided flexible capacitor in which PVDF is used as the ferroelectric layer and the carrier layer. Results show that the nanodevices perform with high repeatability and stability. Self-peel-off transfer is a viable preparation strategy for the design and fabrication of flexible, ultrathin, and light-weight nanodevices.
    Citation
    Tai Y, Lubineau G (2016) “Self-Peel-Off” Transfer Produces Ultrathin Polyvinylidene-Fluoride-Based Flexible Nanodevices. Advanced Science: 1600370. Available: http://dx.doi.org/10.1002/advs.201600370.
    Sponsors
    This research was supported by the King Abdullah University of Science and Technology (KAUST) baseline research funds. The authors are grateful to KAUST for its financial support.
    Publisher
    Wiley
    Journal
    Advanced Science
    DOI
    10.1002/advs.201600370
    Additional Links
    http://onlinelibrary.wiley.com/doi/10.1002/advs.201600370/abstract
    ae974a485f413a2113503eed53cd6c53
    10.1002/advs.201600370
    Scopus Count
    Collections
    Articles; Physical Science and Engineering (PSE) Division; Mechanical Engineering Program

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