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    Towards versatile and sustainable hydrogen production via electrocatalytic water splitting: Electrolyte engineering

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    Shinagawa_et_al-2016-ChemSusChem.pdf
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    Description:
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    Type
    Article
    Authors
    Shinagawa, Tatsuya cc
    Takanabe, Kazuhiro cc
    KAUST Department
    Catalysis for Energy Conversion (CatEC)
    Chemical Science Program
    KAUST Catalysis Center (KCC)
    Physical Science and Engineering (PSE) Division
    Date
    2017-03-09
    Online Publication Date
    2017-03-09
    Print Publication Date
    2017-04-10
    Permanent link to this record
    http://hdl.handle.net/10754/622743
    
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    Abstract
    Recent advances in power generation from renewable resources necessitate conversion of electricity to chemicals and fuels in an efficient manner. The electrocatalytic water splitting is one of the most powerful and widespread technologies. The development of highly efficient, inexpensive, flexible and versatile water electrolysis devices is desired. This review discusses the significance and impact of the electrolyte on electrocatalytic performance. Depending on the circumstances where water splitting reaction is conducted, required solution conditions such as the identity and molarity of ions may significantly differ. Quantitative understanding of such electrolyte properties on electrolysis performance is effective to facilitate developing efficient electrocatalytic systems. The electrolyte can directly participate in reaction schemes (kinetics), electrode stability, and/or indirectly impacts the performance by influencing concentration overpotential (mass transport). This review aims to guide fine-tuning of the electrolyte properties, or electrolyte engineering, for (photo)electrochemical water splitting reactions.
    Citation
    Shinagawa T, Takanabe K (2016) Towards versatile and sustainable hydrogen production via electrocatalytic water splitting: Electrolyte engineering. ChemSusChem. Available: http://dx.doi.org/10.1002/cssc.201601583.
    Sponsors
    The research reported in this work was supported by the King Abdullah University of Science and Technology (KAUST). Cover figure was produced by Ivan Gromicho, scientific illustrator at KAUST.
    Publisher
    Wiley
    Journal
    ChemSusChem
    DOI
    10.1002/cssc.201601583
    Additional Links
    http://onlinelibrary.wiley.com/doi/10.1002/cssc.201601583/abstract
    ae974a485f413a2113503eed53cd6c53
    10.1002/cssc.201601583
    Scopus Count
    Collections
    Articles; Physical Science and Engineering (PSE) Division; Chemical Science Program; KAUST Catalysis Center (KCC)

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