Inorganic Lead Halide Perovskite Single Crystals: Phase-Selective Low-Temperature Growth, Carrier Transport Properties, and Self-Powered Photodetection

Type
Article
Authors
Saidaminov, Makhsud I. cc
Haque, Mohammed
Almutlaq, Jawaher cc
Sarmah, Smritakshi P.
Miao, Xiaohe
Begum, Raihana
Zhumekenov, Ayan A.
Dursun, Ibrahim cc
Cho, Nam Chul
Banavoth, Murali cc
Mohammed, Omar F. cc
Wu, Tao cc
Bakr, Osman cc
KAUST Department
Physical Sciences and Engineering (PSE) Division
Materials Science and Engineering Program
Imaging and Characterization Core Lab
Date
2016-12-06

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Abstract
A rapid, low-temperature, and solution-based route is developed for growing large-sized cesium lead halide perovskite single crystals under ambient conditions. An ultralow minority carrier concentration was measured in CsPbBr3 (≈108 holes per cm3, much lower than in any other lead halide perovskite and crystalline silicon), which enables to realize self-powered photodetectors with a high ON/OFF ratio (105).
Citation
Saidaminov MI, Haque MA, Almutlaq J, Sarmah S, Miao X-H, et al. (2016) Inorganic Lead Halide Perovskite Single Crystals: Phase-Selective Low-Temperature Growth, Carrier Transport Properties, and Self-Powered Photodetection. Advanced Optical Materials: 1600704. Available: http://dx.doi.org/10.1002/adom.201600704.
Sponsors
M.I.S. and M.A.H. contributed equally to this work. This work was supported by KAUST.
Publisher
Wiley-Blackwell
Journal
Advanced Optical Materials
ISSN
2195-1071
DOI
10.1002/adom.201600704
Handle URI
http://hdl.handle.net/10754/622667
Additional Links
http://onlinelibrary.wiley.com/doi/10.1002/adom.201600704/full
Collections
Articles; Advanced Nanofabrication, Imaging and Characterization Core Lab; Physical Sciences and Engineering (PSE) Division; Materials Science and Engineering Program