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    Hybrid Perovskite Thin-Film Photovoltaics: In Situ Diagnostics and Importance of the Precursor Solvate Phases

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    Type
    Article
    Authors
    Munir, Rahim cc
    Sheikh, Arif D. cc
    Abdelsamie, Maged cc
    Hu, Hanlin cc
    Yu, Liyang
    Zhao, Kui cc
    Kim, Taesoo cc
    El Tall, Omar
    Li, Ruipeng
    Smilgies, Detlef-M. cc
    Amassian, Aram cc
    KAUST Department
    Analytical Chemistry Core Lab
    KAUST Solar Center (KSC)
    Material Science and Engineering Program
    Organic Electronics and Photovoltaics Group
    Physical Science and Engineering (PSE) Division
    Solids
    Date
    2016-11-07
    Online Publication Date
    2016-11-07
    Print Publication Date
    2017-01
    Permanent link to this record
    http://hdl.handle.net/10754/622108
    
    Metadata
    Show full item record
    Abstract
    Solution-processed hybrid perovskite semiconductors attract a great deal of attention, but little is known about their formation process. The one-step spin-coating process of perovskites is investigated in situ, revealing that thin-film formation is mediated by solid-state precursor solvates and their nature. The stability of these intermediate phases directly impacts the quality and reproducibility of thermally converted perovskite films and their photovoltaic performance.
    Citation
    Munir R, Sheikh AD, Abdelsamie M, Hu H, Yu L, et al. (2016) Hybrid Perovskite Thin-Film Photovoltaics: In Situ Diagnostics and Importance of the Precursor Solvate Phases. Advanced Materials. Available: http://dx.doi.org/10.1002/adma.201604113.
    Sponsors
    This work was supported by the Office of Competitive Research Funds under the Competitive Research Grant (round 1) and Academic Excellence Alliance (round 3). CHESS is supported by the NSF & NIH/NIGMS via NSF award DMR-1332208. A.A. is grateful to SABIC for the Career Development SABIC Chair. The authors are thankful to Heno Hwang for using his artistic abilities to design Figure 4 of this report.
    Publisher
    Wiley
    Journal
    Advanced Materials
    DOI
    10.1002/adma.201604113
    Additional Links
    http://onlinelibrary.wiley.com/doi/10.1002/adma.201604113/full
    ae974a485f413a2113503eed53cd6c53
    10.1002/adma.201604113
    Scopus Count
    Collections
    Articles; Analytical Chemistry Core Lab; Physical Science and Engineering (PSE) Division; Material Science and Engineering Program; KAUST Solar Center (KSC)

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