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    Functionalization of Planet-Satellite Nanostructures Revealed by Nanoscopic Localization of Distinct Macromolecular Species

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    Type
    Article
    Authors
    Rossner, Christian
    Roddatis, Vladimir
    Lopatin, Sergei cc
    Vana, Philipp
    KAUST Department
    Core Labs
    Electron Microscopy
    Date
    2016-09-26
    Online Publication Date
    2016-09-26
    Print Publication Date
    2016-11
    Permanent link to this record
    http://hdl.handle.net/10754/621393
    
    Metadata
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    Abstract
    The development of a straightforward method is reported to form hybrid polymer/gold planet-satellite nanostructures (PlSNs) with functional polymer. Polyacrylate type polymer with benzyl chloride in its backbone as a macromolecular tracer is synthesized to study its localization within PlSNs by analyzing the elemental distribution of chlorine. The functionalized nanohybrid structures are analyzed by scanning transmission electron microscopy, electron energy loss spectroscopy, and spectrum imaging. The results show that the RAFT (reversible addition-fragmentation chain transfer) polymers' sulfur containing end groups are colocalized at the gold cores, both within nanohybrids of simple core-shell morphology and within higher order PlSNs, providing microscopic evidence for the affinity of the RAFT group toward gold surfaces. © 2016 WILEY-VCH Verlag GmbH & Co. KGaA., Weinheim.
    Citation
    Rossner C, Roddatis V, Lopatin S, Vana P (2016) Functionalization of Planet-Satellite Nanostructures Revealed by Nanoscopic Localization of Distinct Macromolecular Species. Macromolecular Rapid Communications. Available: http://dx.doi.org/10.1002/marc.201600480.
    Sponsors
    Deutsche Forschungsgemeinschaft[VA226-10/1]
    Fonds der Chemischen Industrie
    Publisher
    Wiley
    Journal
    Macromolecular Rapid Communications
    DOI
    10.1002/marc.201600480
    ae974a485f413a2113503eed53cd6c53
    10.1002/marc.201600480
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