• Login
    View Item 
    •   Home
    • Research
    • Articles
    • View Item
    •   Home
    • Research
    • Articles
    • View Item
    JavaScript is disabled for your browser. Some features of this site may not work without it.

    Browse

    All of KAUSTCommunitiesIssue DateSubmit DateThis CollectionIssue DateSubmit Date

    My Account

    Login

    Quick Links

    Open Access PolicyORCID LibguideTheses and Dissertations LibguideSubmit an Item

    Statistics

    Display statistics

    High Efficiency Inverted Organic Solar Cells with a Neutral Fulleropyrrolidine Electron Collecting Interlayer

    • CSV
    • RefMan
    • EndNote
    • BibTex
    • RefWorks
    Thumbnail
    Name:
    acsami2E6b03974.pdf
    Size:
    1.243Mb
    Format:
    PDF
    Description:
    Accepted Manuscript
    Download
    Type
    Article
    Authors
    Xu, Weidong
    Yan, Congfei
    Kan, Zhipeng
    Wang, Yang
    Lai, Wen-Yong
    Huang, Wei cc
    KAUST Department
    KAUST Solar Center (KSC)
    Physical Science and Engineering (PSE) Division
    Date
    2016-05-26
    Online Publication Date
    2016-05-26
    Print Publication Date
    2016-06-08
    Permanent link to this record
    http://hdl.handle.net/10754/610608
    
    Metadata
    Show full item record
    Abstract
    A novel fulleropyrrolidine derivative, named as FPNOH, was designed, synthesized and utilized as an efficient electron-collecting (EC) layer for inverted organic solar cells (i-OSCs). The grafted diethanolamino-polar moieties can not only trigger its function as an EC interlayer, but also induce orthogonal solubility that guarantees subsequent multi-layer processing without interfacial mixing. A higher power conversion efficiency (PCE) value of 8.34% was achieved for i-OSC devices with ITO/FPNOH EC electrode, compared to that of the sol-gel ZnO based reference devices with an optimized PCE value of 7.92%. High efficiency exceeding 7.7% was still achieved even for the devices with a relatively thick PFNOH film (16.9 nm). It is worthwhile to mention that this kind of material exhibits less thickness dependent performance, in contrast to widely utilized p-type conjugated polyelectrolytes (CPEs) as well as the non-conjugated polyelectrolytes (NCPEs). Further investigation on illuminating intensity dependent parameters revealed the role of FPNOH in reducing interfacial traps-induced recombination at ITO/active layer interface.
    Citation
    High Efficiency Inverted Organic Solar Cells with a Neutral Fulleropyrrolidine Electron Collecting Interlayer 2016 ACS Applied Materials & Interfaces
    Sponsors
    We acknowledge financial support of the National Key Basic Research Program of China (973 Program, 2014CB648300), the National Natural Science Foundation of China (21422402, 20904024, 51173081, 61136003), the Natural Science Foundation of Jiangsu Province (BK20140060, BK20130037, BM2012010), Program for Jiangsu Specially-Appointed Professors (RK030STP15001), Program for New Century Excellent Talents in University (NCET-13-0872), Specialized Research Fund for the Doctoral Program of Higher Education (20133223110008, and 20113223110005), the Synergetic Innovation Center for Organic Electronics and Information Displays, the Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD), the NUPT "1311 Project", the Six Talent Plan (2012XCL035), the 333 Project (BRA2015374) and the Qing Lan Project of Jiangsu Province.
    Publisher
    American Chemical Society (ACS)
    Journal
    ACS Applied Materials & Interfaces
    DOI
    10.1021/acsami.6b03974
    PubMed ID
    27197741
    Additional Links
    http://pubs.acs.org/doi/abs/10.1021/acsami.6b03974
    ae974a485f413a2113503eed53cd6c53
    10.1021/acsami.6b03974
    Scopus Count
    Collections
    Articles; Physical Science and Engineering (PSE) Division; KAUST Solar Center (KSC)

    entitlement

    Related articles

    • Well-defined star-shaped conjugated macroelectrolytes as efficient electron-collecting interlayer for inverted polymer solar cells.
    • Authors: Xu W, Kan Z, Ye T, Zhao L, Lai WY, Xia R, Lanzani G, Keivanidis PE, Huang W
    • Issue date: 2015 Jan 14
    • Sulfonate-Conjugated Polyelectrolytes as Anode Interfacial Layers in Inverted Organic Solar Cells.
    • Authors: Lassi E, Squeo BM, Sorrentino R, Scavia G, Mrakic-Sposta S, Gussoni M, Vercelli B, Galeotti F, Pasini M, Luzzati S
    • Issue date: 2021 Feb 2
    • Improvement of Charge Collection and Performance Reproducibility in Inverted Organic Solar Cells by Suppression of ZnO Subgap States.
    • Authors: Wu B, Wu Z, Yang Q, Zhu F, Ng TW, Lee CS, Cheung SH, So SK
    • Issue date: 2016 Jun 15
    • Air-stable efficient inverted polymer solar cells using solution-processed nanocrystalline ZnO interfacial layer.
    • Authors: Tan MJ, Zhong S, Li J, Chen Z, Chen W
    • Issue date: 2013 Jun 12
    • Organic/Organic Cathode Bi-Interlayers Based on a Water-Soluble Nonconjugated Polymer and an Alcohol-Soluble Conjugated Polymer for High Efficiency Inverted Polymer Solar Cells.
    • Authors: Cai P, Jia H, Chen J, Cao Y
    • Issue date: 2015 Dec 23
    DSpace software copyright © 2002-2022  DuraSpace
    Quick Guide | Contact Us | KAUST University Library
    Open Repository is a service hosted by 
    Atmire NV
     

    Export search results

    The export option will allow you to export the current search results of the entered query to a file. Different formats are available for download. To export the items, click on the button corresponding with the preferred download format.

    By default, clicking on the export buttons will result in a download of the allowed maximum amount of items. For anonymous users the allowed maximum amount is 50 search results.

    To select a subset of the search results, click "Selective Export" button and make a selection of the items you want to export. The amount of items that can be exported at once is similarly restricted as the full export.

    After making a selection, click one of the export format buttons. The amount of items that will be exported is indicated in the bubble next to export format.