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    Syntheses, characterizations, and catalytic activities of mesostructured aluminophosphates with tailorable acidity assembled with various preformed zeolite nanoclusters

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    Type
    Article
    Authors
    Suo, Hongri
    Zeng, Shangjing
    Wang, Runwei cc
    Zhang, Zongtao
    Qiu, Shilun
    KAUST Grant Number
    CRG-1-2012-LAI-009
    Date
    2015-02-25
    Online Publication Date
    2015-02-25
    Print Publication Date
    2015-04
    Permanent link to this record
    http://hdl.handle.net/10754/599829
    
    Metadata
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    Abstract
    © 2015, Springer Science+Business Media New York. A series of ordered hexagonal mesoporous zeolites have been successfully synthesized by the assembly of various preformed aluminosilicates zeolite (MFI, FAU, BEA etc.) with surfactants (cetyltrimethylammonium chloride) under hydrothermal conditions. These unique samples were further characterized by X-ray diffraction, transmission electron microscopy, N2 adsorption, infrared spectroscopy. Characterization results showed that these samples contain primary and secondary structural building units of various zeolites, which may be responsible for their distinguished acidic strength, suggesting that the acidic strength of these mesoporous silicoaluminophosphates could be tailored and controlled. Furthermore, the prepared samples were catalytically active in the cracking of cumene.
    Citation
    Suo H, Zeng S, Wang R, Zhang Z, Qiu S (2015) Syntheses, characterizations, and catalytic activities of mesostructured aluminophosphates with tailorable acidity assembled with various preformed zeolite nanoclusters. J Porous Mater 22: 529–536. Available: http://dx.doi.org/10.1007/s10934-015-9923-y.
    Sponsors
    This work was supported by National Natural Science Foundation of China (21390394), the National Basic Research Program of China (2012CB821700, 2011CB808703), NSFC (212611 30584, 91022030), "111" project (B07016), Award Project of KAUST (CRG-1-2012-LAI-009) and Ministry of Education, Science and Technology Development Center Project (20120061130012).
    Publisher
    Springer Nature
    Journal
    Journal of Porous Materials
    DOI
    10.1007/s10934-015-9923-y
    ae974a485f413a2113503eed53cd6c53
    10.1007/s10934-015-9923-y
    Scopus Count
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    Publications Acknowledging KAUST Support

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