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    Strong and Stable Doping of Carbon Nanotubes and Graphene by MoO x for Transparent Electrodes

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    Type
    Article
    Authors
    Hellstrom, Sondra L.
    Vosgueritchian, Michael
    Stoltenberg, Randall M.
    Irfan, Irfan
    Hammock, Mallory
    Wang, Yinchao Bril
    Jia, Chuancheng
    Guo, Xuefeng
    Gao, Yongli
    Bao, Zhenan
    KAUST Grant Number
    KUS-C1-015-21
    Date
    2012-06-13
    Online Publication Date
    2012-06-13
    Print Publication Date
    2012-07-11
    Permanent link to this record
    http://hdl.handle.net/10754/599748
    
    Metadata
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    Abstract
    MoO x has been used for organic semiconductor doping, but it had been considered an inefficient and/or unstable dopant. We report that MoO x can strongly and stably dope carbon nanotubes and graphene. Thermally annealed MoO x-CNT composites can form durable thin film electrodes with sheet resistances of 100 ω/sq at 85% transmittance plain and 85 ω/sq at 83% transmittance with a PEDOT:PSS adlayer. Sheet resistances change less than 10% over 20 days in ambient and less than 2% with overnight heating to 300 °C in air. The MoO x can be easily deposited either by thermal evaporation or from solution-based precursors. Excellent stability coupled with high conductivity makes MoO x-CNT composites extremely attractive candidates for practical transparent electrodes. © 2012 American Chemical Society.
    Citation
    Hellstrom SL, Vosgueritchian M, Stoltenberg RM, Irfan I, Hammock M, et al. (2012) Strong and Stable Doping of Carbon Nanotubes and Graphene by MoO x for Transparent Electrodes . Nano Lett 12: 3574–3580. Available: http://dx.doi.org/10.1021/nl301207e.
    Sponsors
    S.L.H. and Z.B. would like to thank the Stanford University Global Climate and Energy Project (GCEP) for partial funding. This publication was partially based on work supported by the Center for Advanced Molecular Photovoltaics (Award No. KUS-C1-015-21) made by King Abdullah University of Science and Technology (KAUST).
    Publisher
    American Chemical Society (ACS)
    Journal
    Nano Letters
    DOI
    10.1021/nl301207e
    PubMed ID
    22694046
    ae974a485f413a2113503eed53cd6c53
    10.1021/nl301207e
    Scopus Count
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