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    Rotary Bed Reactor for Chemical-Looping Combustion with Carbon Capture. Part 1: Reactor Design and Model Development

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    Type
    Article
    Authors
    Zhao, Zhenlong cc
    Chen, Tianjiao
    Ghoniem, Ahmed F.
    Date
    2012-12-12
    Online Publication Date
    2012-12-12
    Print Publication Date
    2013-01-17
    Permanent link to this record
    http://hdl.handle.net/10754/599539
    
    Metadata
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    Abstract
    Chemical-looping combustion (CLC) is a novel and promising technology for power generation with inherent CO2 capture. Currently, almost all of the research has been focused on developing CLC-based interconnected fluidized-bed reactors. In this two-part series, a new rotary reactor concept for gas-fueled CLC is proposed and analyzed. In part 1, the detailed configuration of the rotary reactor is described. In the reactor, a solid wheel rotates between the fuel and air streams at the reactor inlet and exit. Two purging sectors are used to avoid the mixing between the fuel stream and the air stream. The rotary wheel consists of a large number of channels with copper oxide coated on the inner surface of the channels. The support material is boron nitride, which has high specific heat and thermal conductivity. Gas flows through the reactor at elevated pressure, and it is heated to a high temperature by fuel combustion. Typical design parameters for a thermal capacity of 1 MW have been proposed, and a simplified model is developed to predict the performances of the reactor. The potential drawbacks of the rotary reactor are also discussed. © 2012 American Chemical Society.
    Citation
    Zhao Z, Chen T, Ghoniem AF (2013) Rotary Bed Reactor for Chemical-Looping Combustion with Carbon Capture. Part 1: Reactor Design and Model Development. Energy Fuels 27: 327–343. Available: http://dx.doi.org/10.1021/ef3014103.
    Sponsors
    This study is financially supported by a grant from the MASDAR Institute of Science and Technology and the King Abdullah University of Science and Technology (KAUST) Investigator Award.
    Publisher
    American Chemical Society (ACS)
    Journal
    Energy & Fuels
    DOI
    10.1021/ef3014103
    ae974a485f413a2113503eed53cd6c53
    10.1021/ef3014103
    Scopus Count
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    Publications Acknowledging KAUST Support

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