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    Perovskite Thin Films via Atomic Layer Deposition

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    Type
    Article
    Authors
    Sutherland, Brandon R.
    Hoogland, Sjoerd
    Adachi, Michael M.
    Kanjanaboos, Pongsakorn
    Wong, Chris T. O.
    McDowell, Jeffrey J.
    Xu, Jixian
    Voznyy, Oleksandr cc
    Ning, Zhijun
    Houtepen, Arjan J.
    Sargent, Edward H. cc
    KAUST Grant Number
    KUS-11-009-21
    Date
    2014-10-30
    Online Publication Date
    2014-10-30
    Print Publication Date
    2015-01
    Permanent link to this record
    http://hdl.handle.net/10754/599170
    
    Metadata
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    Abstract
    © 2014 Wiley-VCH Verlag GmbH & Co. KGaA. (Graph Presented) A new method to deposit perovskite thin films that benefit from the thickness control and conformality of atomic layer deposition (ALD) is detailed. A seed layer of ALD PbS is place-exchanged with PbI2 and subsequently CH3NH3PbI3 perovskite. These films show promising optical properties, with gain coefficients of 3200 ± 830 cm-1.
    Citation
    Sutherland BR, Hoogland S, Adachi MM, Kanjanaboos P, Wong CTO, et al. (2014) Perovskite Thin Films via Atomic Layer Deposition. Advanced Materials 27: 53–58. Available: http://dx.doi.org/10.1002/adma.201403965.
    Sponsors
    This publication is based in part on work supported by an award (KUS-11-009-21) from the King Abdullah University of Science and Technology (KAUST), by the Ontario Research Fund Research Excellence Program and by the Natural Sciences and Engineering Research Council (NSERC) of Canada. The authors thank Cambridge Nanotech, Fritz Prinz, and Orlando Trejo for their advice on ALD PbS film fabrication. The authors thank L.T. Kunneman for his assistance in the data analysis of the transient absorption measurements. The authors also thank M. Yuan, H. Dong, R. Wolowiec, and D. Kopilovic for their help during the course of the study.
    Publisher
    Wiley
    Journal
    Advanced Materials
    DOI
    10.1002/adma.201403965
    PubMed ID
    25359103
    ae974a485f413a2113503eed53cd6c53
    10.1002/adma.201403965
    Scopus Count
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