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    Ordered Nanopillar Structured Electrodes for Depleted Bulk Heterojunction Colloidal Quantum Dot Solar Cells

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    Type
    Article
    Authors
    Kramer, Illan J. cc
    Zhitomirsky, David
    Bass, John D.
    Rice, Philip M.
    Topuria, Teya
    Krupp, Leslie
    Thon, Susanna M.
    Ip, Alexander H.
    Debnath, Ratan
    Kim, Ho-Cheol
    Sargent, Edward H. cc
    KAUST Grant Number
    KUS-11-009-21
    Date
    2012-03-30
    Online Publication Date
    2012-03-30
    Print Publication Date
    2012-05-02
    Permanent link to this record
    http://hdl.handle.net/10754/599110
    
    Metadata
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    Abstract
    A bulk heterojunction of ordered titania nanopillars and PbS colloidal quantum dots is developed. By using a pre-patterned template, an ordered titania nanopillar matrix with nearest neighbours 275 nm apart and height of 300 nm is fabricated and subsequently filled in with PbS colloidal quantum dots to form an ordered depleted bulk heterojunction exhibiting power conversion efficiency of 5.6%. Copyright © 2012 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
    Citation
    Kramer IJ, Zhitomirsky D, Bass JD, Rice PM, Topuria T, et al. (2012) Ordered Nanopillar Structured Electrodes for Depleted Bulk Heterojunction Colloidal Quantum Dot Solar Cells. Advanced Materials 24: 2315–2319. Available: http://dx.doi.org/10.1002/adma.201104832.
    Sponsors
    This publication is based on work in part supported by Award No. KUS-11-009-21, made by King Abdullah University of Science and Technology (KAUST), the Ontario Research Fund Research in Excellence Program and the Natural Sciences and Engineering Research Council (NSERC) of Canada. We thank Angstrom Engineering and Innovative Technologies for useful discussions regarding material deposition methods and control of glovebox environment, respectively. I.J.K., D.Z., A. H. I. and R. D. acknowledge the financial support through the Ontario Graduate Scholarship, the NSERC CGS D Scholarship, the Queen Elizabeth II Graduate Scholarship in Science and Technology and the MITACS Elevate Strategic Fellowship, respectively. H-C. K. thanks Eugene Delenia (at IBM Almaden Research Center) for TEM sample preparation. He also thanks Robert Miller (IBM), Campbell Scott (IBM) and Fahhad Alharbi (King Abdulaziz City of Science and Technology) and useful discussions. The authors would also like to acknowledge the technical assistance and scientific guidance of E. Palmiano, R. Wolowiec and D. Kopilovic.
    Publisher
    Wiley
    Journal
    Advanced Materials
    DOI
    10.1002/adma.201104832
    PubMed ID
    22467240
    ae974a485f413a2113503eed53cd6c53
    10.1002/adma.201104832
    Scopus Count
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