Show simple item record

dc.contributor.authorPeppin, S. S. L.
dc.contributor.authorSpannuth, M. J.
dc.contributor.authorWettlaufer, J. S.
dc.date.accessioned2016-02-25T13:52:26Z
dc.date.available2016-02-25T13:52:26Z
dc.date.issued2009-03-04
dc.identifier.citationPeppin SSL, Spannuth MJ, Wettlaufer JS (2009) Onsager Reciprocity in Premelting Solids. J Stat Phys 134: 701–708. Available: http://dx.doi.org/10.1007/s10955-009-9699-z.
dc.identifier.issn0022-4715
dc.identifier.issn1572-9613
dc.identifier.doi10.1007/s10955-009-9699-z
dc.identifier.urihttp://hdl.handle.net/10754/599077
dc.description.abstractThe diffusive motion of foreign particles dispersed in a premelting solid is analyzed within the framework of irreversible thermodynamics. We determine the mass diffusion coefficient, thermal diffusion coefficient and Soret coefficient of the particles in the dilute limit, and find good agreement with experimental data. In contrast to liquid suspensions, the unique nature of premelting solids allows us to derive an expression for the Dufour coefficient and independently verify the Onsager reciprocal relation coupling diffusion to the flow of heat. © 2009 Springer Science+Business Media, LLC.
dc.description.sponsorshipThis research was supported by the Department of Energy (DE-FG02-05ER15741) and by the U. S. National Science Foundation (OPP0440841). S. S. L. P. acknowledges support from the King Abdullah University of Science and Technology (KAUST), Award No. KUK-C1-013-04. M. J. S. acknowledges support from a U. S. National Science Foundation Graduate Research Fellowship. J. S. W. is grateful for support from the Wenner-Gren Foundation, the Royal Institute of Technology and NORDITA all in Stockholm.
dc.publisherSpringer Nature
dc.subjectColloids
dc.subjectDiffusion
dc.subjectDufour effect
dc.subjectPremelting
dc.subjectReciprocity
dc.subjectSoret effect
dc.subjectSurface phase transitions
dc.titleOnsager Reciprocity in Premelting Solids
dc.typeArticle
dc.identifier.journalJournal of Statistical Physics
dc.contributor.institutionYale University, New Haven, United States
dc.contributor.institutionUniversity of Oxford, Oxford, United Kingdom
dc.contributor.institutionNordisk Institut for Teoretisk Atomtysik, Stockholm, Sweden
kaust.grant.numberKUK-C1-013-04
dc.date.published-online2009-03-04
dc.date.published-print2009-02


This item appears in the following Collection(s)

Show simple item record